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Y. Liu,S. Hashimoto,K. Yasumoto,K. Takei,M. Mori,Y. Funahashi,Y. Fijishiro,A. Hirano,Y. Takeda 한국물리학회 2009 Current Applied Physics Vol.9 No.11
The catalytic activity of the La0.6Sr0.4CoxFe1-xO3-δ (x = 0.2) perovskite cathode was significantly improved by introducing Ag. This strongly depends on the particle size of Ag that relates to the synthesis route. The Ag particles in nano-range were in situ incorporated into the La0.6Sr0.4Co0.2Fe0.8O3-δ based cathode using a novel infiltration. The functional cathode was successfully operated on the anode-supported cell with a ceria thin-electrolyte resulting in a higher cell output at 500 ℃. Durability of the cell was evaluated within a short-term period. The catalytic activity of the La0.6Sr0.4CoxFe1-xO3-δ (x = 0.2) perovskite cathode was significantly improved by introducing Ag. This strongly depends on the particle size of Ag that relates to the synthesis route. The Ag particles in nano-range were in situ incorporated into the La0.6Sr0.4Co0.2Fe0.8O3-δ based cathode using a novel infiltration. The functional cathode was successfully operated on the anode-supported cell with a ceria thin-electrolyte resulting in a higher cell output at 500 ℃. Durability of the cell was evaluated within a short-term period.
Two competing soft modes and an unusual phase transition in the stuffed tridymite-type oxideBaAl2O4
Ishii, Y.,Mori, S.,Nakahira, Y.,Moriyoshi, C.,Park, J.,Kim, B. G.,Moriwake, H.,Taniguchi, H.,Kuroiwa, Y. American Physical Society 2016 Physical Review B Vol.93 No.13
<P>We investigated the structural phase transition of BaAl2O4, which has a network structure with corner-sharing AlO4 tetrahedra, via synchrotron x-ray thermal diffuse scattering measurements and first-principles calculations. BaAl2O4 shows the structural phase transition at T-C = 451.4 K from the P6(3)22 parent crystal structure to the low-temperature superstructure with a cell volume of 2a x 2b x c. This phase transition is unusual, in which two energetically competing phonon modes at M and K points soften simultaneously. When approaching T-C from above, the K-point mode appears first. However, this K-point mode is overcome by the later-developed M-point mode. The thermal diffuse scattering intensities from both modes increase sharply at T-C; therefore, both modes soften simultaneously. The first-principles calculations demonstrate that the M-point mode is electrostatically more preferable than the K-point mode and determines the eventual low-temperature structure, although these two modes are competing energetically. This competition is characteristic of BaAl2O4, which is ascribed to the structurally flexible network structure of this compound.</P>
Structural Changes and Microstructures of Ba1−xSrxAl2O4 for 0 < x < 0.4
E. Tanaka,Y. Ishii,H. Tsukasaki,S. Mori,M. Osada,H. Taniguchi,Y. Sato,Y. Kubota 한국물리학회 2015 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.66 No.9
We have investigated the structural changes and the microstructures of Ba1−xSrxAl2O4 for 0 < x < 0.4 by using transmission electron microscope (TEM) and synchrotron radiation powder X-ray diffraction experiments. The TEM experiments revealed the existence of a structural phase boundary at approximately x = 0.1, at which the superlattice reflection spots at the 1/2 0 0 −type positions change into diffuse streaks along three equivalent <110> directions in the hexagonal structure. In addition, real-space images of Ba1−xSrxAl2O4 for 0 < x < 0.4 reveal that BaAl2O4 should be characterized as a modulated structure with triple-q modulation vectors along the <100> directions and on the other hand, Ba1−xSrxAl2O4 for 0.1 < x < 0.4 be characterized as an intermediate (precursor) state with a rigid unit mode due to structural instability. These experimental results implied that the partial substitution of Sr2+ for Ba2+ should suppress a structural instability due to the AlO4 tetrahedral network and decrease the structural phase transition temperature.
Characterization of an Intense Laser-Produced Preformed Plasma for Proton Generation
A Sagisaka,A. Noda,A. Fukumi,A. Yogo,A. S. Pirozhkov,H. Daido,K. Nemoto,K. Ogura,M. Nishiuchi,M. Mori,M. Kado,S. Orimo,S. Nakamura,T. Nayuki,T. Shirai,T. Fujii,Y. Oishi,Y. Hayashi,Y. Iwashita,Z. Li 한국물리학회 2007 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.51 No.I
High-energy protons are generated with a 3-μm-thick tantalum target irradiated with a highintensity laser under the preformed plasma condition. We observe the electron density distributions of preformed plasmas with two-color probe beams as interferometers. The preformed plasma at the front side of the target is generated by pre-pulses of a high-intensity Ti:sapphire laser. In this preformed plasma condition, the maximum proton enegy is 900 keV. The half angle of the generated proton beam (>500 keV) is about 10.
Structural phase transitions and dielectric anomaly in YFe2O4-δ
Y. Horibe,K. Kishimoto,N. Ikeda,S. Mori 한국물리학회 2005 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.46 No.1
We examined structural changes related to charge ordering (CO) in the temperature window between 100 K and room temperature (RT) in YFe2O4 by transmission electron microscopy. Characteristic diuse scattering elongated along the [001] direction through the (1/3 1/3 0)-type reciprocal positions was found at RT, which is related to the microdomains due to the CO with a size of 10 { 20 nm. In addition, it was also found that the superlattice structures characterized by the (1/3 { 1/3 + 0)-type modulation vector, which should be due to the vacancy ordering,coexist with the microdomains due to the CO. On the other hand, in stoichimetric YFe2O4, we found temperature variations of the superlattice structures on warming from 100 K, which should be strongly related to the dielectric anomalies in YFe2O4.
Mori, K.,Yang, C.Y. Pergamon Press 2016 Tetrahedron Vol.72 No.30
<P>Seven new methyl-branched hydrocarbons were synthesized, which were the pheromone candidates of the female Korean apricot wasp (Eurytoma maslovskii). They are (Z)-15-methyl-7-nonacosene (1), (Z)-17-methyl-7-hentriacontene (2), 3,7-dimethylheptacosane (3), 8,12-dimethyltriacontane (4), 8,18-dimethyltriacontane (5), 3,7,11-trimethylnonacosane (6), and 3,7,17-trimethylnonacosane (7). All of them were synthesized as stereoisomeric mixtures, employing short and simple routes. Hydrocarbon 7 was synthesized via 4,8-dimethyldecanal (71, tribolure), the red flour beetle pheromone. The hydrocarbons 1,2,3 and 6 were identified by GC-MS analysis as the components (with unknown stereo chemistry) of the female-specific secretion of E. maslovskii. (C) 2016 Elsevier Ltd. All rights reserved.</P>