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Nguyen Le Minh Tri,김지태,Bach Long Giang,T.M. Al Tahtamouni,Pham Thi Huong,이창하,Nguyen Minh Viet,Do Quang Trung 한국공업화학회 2019 Journal of Industrial and Engineering Chemistry Vol.80 No.-
In this study a novel Ag-doped graphitic carbon nitride (g-C3N4) photocatalyst was synthesized and appliedas high efficientmaterial under solarlight towardsemerging antibiotic pollutantin hospital wastewater. Thetetracycline (TC) was chosen as a target pollutant and the content of Ag doping at 3 mmol revealed thehighest photocatalytic degradation efficiency of TC (96.8%) after 120 min under solar light irradiation. Thephotoluminescence and UV–vis analysis confirmed the enhancement of charge separation and transfer inthe graphitic carbon structure after Ag-doping. The removal efficiency of TC using g-C3N4 and Ag-doped g-C3N4 (AgCN) underdark conditions was only 25.6 and 31.8%, respectively. While under solarlight conditions,the removal efficiency of TC increased to 68.3 and 96.8% for g-C3N4 and AgCN, respectively. The reusabilityprocess showed that AgCN displayed extremely high stability after 6 cycles without significant drop inantibiotic degradation efficiency. The application of AgCN was tested for treatment of TC from hospitalwastewater and it showed high removal efficiency of 89.6% within 120 min reaction time. In addition, theintermediatesgeneratedandreductionof total organiccarbon(TOC)duringthephotocatalyticreactionweredetected to support information of possible TC removal mechanism.