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Antiferromagnetic coupling of van der Waals ferromagnetic Fe<sub>3</sub>GeTe<sub>2</sub>
Kim, Dongseuk,Park, Sijin,Lee, Jinhwan,Yoon, Jungbum,Joo, Sungjung,Kim, Taeyueb,Min, Kil-joon,Park, Seung-Young,Kim, Changsoo,Moon, Kyoung-Woong,Lee, Changgu,Hong, Jisang,Hwang, Chanyong IOP Pub 2019 Nanotechnology Vol.30 No.24
<P>Among two-dimensional (2D) layered van der Waals materials, ferromagnetic 2D materials can be useful for compact low-power spintronic applications. One promising candidate material is Fe<SUB>3</SUB>GeTe<SUB>2</SUB> (FGT), which has a strong perpendicular magnetic anisotropy and relatively high Curie temperature. In this study, we confirmed that an oxide layer (O-FGT) naturally forms on top of exfoliated FGT and that an antiferromagnetic coupling (AFC) exists between FGT and O-FGT layers. From a first-principles calculation, oxide formation at the interface of each layer induces an AFC between the layers. An AFC causes a tailed hysteresis loop, where two-magnetization reversal curves are included, and a negative remanence magnetization at a certain temperature range.</P>