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Pengtao Yan,Lei Yan,Sumei Zhao,Zhen Zuo,Xiaoxu Wang,Chenglin Wang,Meiling Hou 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2019 NANO Vol.14 No.8
A graphene-based composite with high electrochemical performance for supercapacitor applications is fabricated by introducing nanoscale carbide-derived carbon (NCDC) into the fluorine-doped graphene (FG). The incorporation of fluorine can increase the specific capacitance of graphene by providing more pseudocapacitance, whereas the introduction of NCDC into the FG/NCDC composite offers high specific surface area (SSA) (up to 1317 m2 g -1) and hierarchical pore structure, resulting in an enhanced electric double layer capacitance. Due to the synergistic effect of pseudocapacitance and electric double layer capacitance, the specific capacitance of FG/NCDC composite can reach 321 F g -1 at a scan rate of 5 mV s -1 in aqueous electrolyte. Notably, the specific capacitance of the FG/NCDC composite is very stable during long-term cyclic tests, with no significant degradation after 10,000 cycles. Due to its excellent supercapacitive performance, the FG/NCDC composite can be considered as a promising electrode material for high-performance supercapacitors.
Zhen Zuo,Yulin Yang,Pengtao Yan,Laizhou Song,Xin Jin 한국섬유공학회 2022 Fibers and polymers Vol.23 No.6
Polyethersulfone (PES)/polytetrafluoroethylene (PTFE) based composite were prepared with the nanofiller oforganic montmorillonite (OMMT). Compared with original OMMT, the interlayer spacing of OMMT in nanocomposites wasdecreased from 3.47 nm to 1.35 nm, attributing to the decomposition of interlayer quaternary ammonium salt. OMMTnanofiller was favorable to improve the thermal stability and abrasion resistance of PES/PTFE compounds. The preferablewear property of OMMT/PES/PTFE composite was mainly ascribed to the load bearing capacity of OMMT on the wornsurface of polymer composites. The OMMT/PES/PTFE compound with 10 wt% OMMT exhibited the lowest wear rate,owing to its densification morphology. Because of the absence of PTFE transfer film, the friction coefficient of OMMT/PES/PTFE compound with 10 wt% OMMT were higher than those of PTFE and PES/PTFE compounds.
High-Performance Supercapacitor based on the NaOH Activated D-Glucose Derived Carbon
Chao Wu,Jiang Xu,Jianning Ding,Ningyi Yuan,Pengtao Yan,Ruijun Zhang,Huihan Liu 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2016 NANO Vol.11 No.7
In this work, a mechanism of catalytic graphitization of D-glucose derived carbon during NaOH activation process is disclosed. The catalytic graphitization is caused by sodium atom, which is produced in the reaction between NaOH and carbon. Due to the combined action of activation and catalytic graphitization resulting from the NaOH, the activated D-glucose derived carbon behaves as a hierarchical micro- and meso-porous structure and has high electrical conductivity. Electrochemical investigations demonstrate that the activated sample exhibits an outstanding rate capability (70% of capacity retention even at a scan rate of 2 V s-1) and high specific capacitance (106 F g-1) in 6 M KOH aqueous electrolyte, which makes it a promising electrode material for high-power supercapacitors.
Wang Yongpeng,Wang Heng,Zhang Qingwen,Zhang Yingyuan,Yan Pengtao,Liu Mengzhu,Zhang Haibo 한국화학공학회 2023 Korean Journal of Chemical Engineering Vol.40 No.8
Multi-walked carbon nanotube (MWCNT)/poly(aryl ether ketone) networks cross-linked by Diels-Alder cycloaddition possess outstanding mechanical and rheological properties. Poly(aryl ether ketone) containing pendant furan (PAEK-Fu) was synthesized, which had excellent thermal and mechanical properties, and a series of cross-linked materials with reversible covalent cross-linked crosslinking network were synthesized through a furan/MWCNTs Diels-Alder (D-A) reaction between PAEK-Fu and MWCNTs. Thermal and mechanical properties for MWCNT/PAEK-Fu composites were studied, and after crosslinking, MWCNT/PAEK-Fu composites exhibited good flexibility and resistance against organic solvents. After heating to 180 °C, the cross-linked MWCNT/PAEK-Fu composite membranes could be dissolved in NMP. This work demonstrates that the poly(aryl ether ketone)s can be made into recyclable thermoset materials using the concept of associative dynamic bonding. Given the dramatically increasing interest in environmentally sustainable materials, this MWCNT/poly(aryl ether ketone) interaction mode provides a robust approach to high performance engineering plastics with improved performance compared with the thermoplastic counterparts.