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Kang, Hongkyu,Lee, Jinho,Jung, Suhyun,Yu, Kilho,Kwon, Sooncheol,Hong, Soonil,Kee, Seyoung,Lee, Seongyu,Kim, Dongwon,Lee, Kwanghee The Royal Society of Chemistry 2013 Nanoscale Vol.5 No.23
<P>Vertically self-assembled bilayers with an interfacial bottom layer and a photoactive top layer are demonstrated via a single coating step of a blend composed of an amine-containing nonconjugated polyelectrolyte (NPE) and an organic electron donor-acceptor bulk heterojunction composite. The self-assembled NPE layer reduces the work function of an indium tin oxide (ITO) cathode, which leads to efficient inverted organic solar cells without any additional interface engineering of the ITO.</P>
Kang, Hongkyu,Hong, Soonil,Lee, Jongjin,Lee, Kwanghee WILEY‐VCH Verlag 2012 ADVANCED MATERIALS Vol.24 No.22
<P>A highly efficient, flexible polymer inverted solar cell is fabricated by K. Lee and co‐workers from various colored inks. In the image, an enlarged chemical structure of the interface between an indium tin oxide (ITO) cathode (sky‐blue) and a nonconjugated polyelectrolyte (white) is shown. The authors focus in particular on the ionic self‐assembling nature of these novel interfacial materials, achieved via dipole interactions, which dramatically reduce the ITO workfunction. These mechanisms are illustrated schematically on page 3005. </P>