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Surfactant-treated graphene oxide in organic solvents and its application in photovoltaic cells
Yishan Wang,Shengyi Yang,Haowei Wang,Li Zhang,Haijuan Cheng,Bo He,Weile Li,Bingsuo Zou 한국물리학회 2017 Current Applied Physics Vol.17 No.3
In this paper, a simple and non-poisonous “surfactant treatment” method to prepare graphene oxide (GO) in organic solvents with good dispersibility was presented. As the surfactant molecules, didodecyldimethyla-mmonium bromide (DDAB) was attached onto the GO sheets via ionic interactions by mild sonication, the obtained GO:DDAB nanocomposites were then blended into copolymer Poly(3- hexylthiophene-2,5-diyl) (P3HT) [6,6]:-Phenyl C61 butyric acid methyl ester (PC61BM) as the active layer to fabricate bulk-heterojunction (BHJ) organic solar cells ITO/PEDOT:PSS/P3HT:PC61BM:(GO:DDAB)/ Ca/Al. The concentration of GO:DDAB in the active layer, a maximum power conversion efficiency (PCE) of 3.67% was obtained by blending 0.5 mg/mL GO:DDAB in the active layer, showing an efficiency increment of 13.35% as compared with that of the control device without doping GO:DDAB. The optimized OPVs with PTB7:PC71BM by adding GO:DDAB shows the PCE of 7.96%. Therefore, it paves a way to get high efficiency organic photovoltaic cells by directly blending surfactant-treated graphene oxide in organic solvent.
Enalapril maleate as a green accelerator for zinc phosphating coating on low-carbon steel
Weishan Wang,Yuqin Tian,Aojue Ke,Haowei Huang,Huifang Shen,Xinya Zhang 한국공업화학회 2023 Journal of Industrial and Engineering Chemistry Vol.120 No.-
In this study, enalapril maleate (EM), a green ingredient of an antihypertensive drug, was selected as anaccelerator for phosphate coating promoting on low-carbon steel. The scanning electron microscope(SEM), X-ray diffraction (XRD), 3D morphologies, coating weight, coating thickness and free acidity(FA) as well as total acidity (TA) were characterized to analyze the coating performance. Copper sulfatetitration, potentiodynamic polarization (PDP) and electrochemical impedance spectroscopy (EIS) wereperformed to evaluate corrosion resistance of phosphate coatings. The DFT computations were appliedto explore the phosphating promoting mechanism. The results show that the EM optimal concentrationis 1.6 g/L which lowers the operating temperature (form 80 ℃ to 40 ℃), generates the smoothest (Ra = 2. 85 lm), the heaviest (28.35 g/cm2) and the thinnest (21.6 lm) coating, and reduces the corrosion ratefrom 1.099 mpy of blank to 0.0246 mpy. The density functional theory (DFT) results confirm that EMadsorbs on low-carbon steel by electrophilic sites (N10) as well as nucleophilic sites (C10), forms nucleatedparticles preferentially and accelerates the growth of crystals. Therefore, EM is a green organic compoundwith high phosphating promotion efficiency which has potential application prospects inindustrial phosphating.
( Jinglan Ou ),( Haowei Wu ),( Qi Wang ),( Yutao Zou ) 한국인터넷정보학회 2014 KSII Transactions on Internet and Information Syst Vol.8 No.10
The frequency spectrum available for the wireless communication is extremely crowded. In order to improve the spectral efficiency, the two-way relay networks have aroused great attention. A simple N<sup>th</sup> best-relay selection criterion for the opportunistic two-way relay networks is proposed, which can be implemented easily by extending the distributed timer technique in practice, since the proposed criterion is mainly based on the channel gains. The outage performance of the proposed relay selection scheme is analyzed under the outdated channel state information (CSI), and a tight closed-form lower bound and asymptotic value of the outage probability over Rayleigh fading channels are obtained. Simulation results demonstrate that the tight closed-form lower bound of the outage probability very closely matches with simulated ones in the whole SNR region, and the asymptotic results provide good tight approximations to the simulation ones, especially in the high SNR region.
Peng Guo,Zhaojie Wang,Hongyu Chen,Shaohui Ge,Chen Chen,Haowei Wang,Jinbao Zhang,Minglei Hua,Shuxian Wei,Xiaoqing Lu 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2019 NANO Vol.15 No.01
The increasing energy crisis promotes the study on novel electrode materials with high performance for supercapacitive storage and energy conversion. Transition metal phosphates have been reported as a potential candidate due to the unique coordination and corresponding electronic structure. Herein, we adopted a facile method for preparing NaCoPO4@C derived from a metal organic framework (MOF) as a bifunctional electrode. ZIF-67 was synthesized before a refluxing process with Na2HPO4 to form a precursor, which is transformed into the final product via calcination in different atmospheres. Specifically, the resultant NaCoPO4@C exhibits a high specific capacitance of 1178.7 F g -1 at a current density of 1 A g -1 for a supercapacitor. An asymmetric supercapacitor (ASC) assembled with active carbon displays a high capacitance of 163.7 F g -1 at 1 A g -1. In addition, as an oxygen evolution reaction (OER) catalyst, the NaCoPO4@C electrode requires only 299 mV to drive a current density of 10 mA cm -2. These results suggest that the rational design of MOF-derived NaCoPO4@C provides a variety of practical applications in electrochemical energy conversion and storage.
Zhou Xuefei,Miao Wei,Cheng Wenxi,Lin Haowei,Lin Haowei,Zheng Hongjuan,Cheng Qiaohuan,Wang Renjie,Yao Chenxue,Liu Xiaobo 한국화학공학회 2023 Korean Journal of Chemical Engineering Vol.40 No.6
A series of poly(arylene ether nitrile) containing versatile carboxyl and sulfonic groups (CSPEN) were magnetically functionalized by ferroferric oxide (Fe3O4), and the obtained magnetic adsorbents (Fe3O4/CSPEN) were used to remove methylene blue (MB) dye from aqueous solution. The systematical characterizations that including scanning electron microscope (SEM), X-ray powder diffractometer (XRD), X-ray photoelectron spectroscopy (XPS), vibrating sample magnetometer (VSM), Fourier transform infrared (FTIR) certified that the Fe3O4/CSPEN possessed versatile functional groups and magnetic separation properties. The batch adsorption studies revealed that the Fe3O4/CSPEN not only displayed high selective adsorption ability for cationic MB in the presence of anionic MO, but also exhibited a removal efficiency as high as 98.2%. Besides, the adsorption kinetics and isotherm matched well with pseudo-second-order model and Langmuir model, respectively, and the maximum adsorption capacity of Fe3O4/CSPEN for MB was 92.029 mg/g. The FTIR and Brunauer-Emmett-Teller (BET) analyses confirmed that the outstanding adsorption capacity of Fe3O4/CSPEN was attributed to their own microporous structure and the electrostatic interaction with MB. Therefore, the modified magnetic adsorbent can be used to selectively remove cationic dye from aqueous solution.
Research on stiffness control of a redundant cable-driven parallel mechanism
Jinshan Yu,Jianguo Tao,Guoxing Wang,Xiao Li,Haowei Wang 대한기계학회 2022 JOURNAL OF MECHANICAL SCIENCE AND TECHNOLOGY Vol.36 No.11
Controlling the stiffness of cable-driven parallel mechanisms (CDPM) is of great significance for improving performance in different tasks. A method for stiffness control of a redundant CDPM is presented in this paper. The stiffness matrix of the redundant CDPM is established. On this basis, considering the effect of coupling stiffness, a complete analytical formula for stiffness in different directions is established. Then, the influence of the vector λ on the stiffness of the CDPM in different directions is analyzed, and a method to control the stiffness of the CDPM through adjusting the vector λ is proposed. To avoid traversing the value of λ in the polygon formed by the set of λ to obtain the appropriate cable tension and keep the cable tension away from the upper and lower limit values, a change path of the vector λ is designed. When the vector λ changes along the path, the stiffness of the mechanism can be changed from the minimum value to the maximum value. This method has high computational efficiency and safety. Finally, the correctness and effectiveness of the stiffness control method are verified by experiments. The stiffness control method proposed in this paper can be used to control the stiffness in different directions, and can also be used for different types of redundant CDPMs.
Hao, Wei,Tian, Pengjiao,Zheng, Mingli,Wang, Huili,Xu, Chuncheng Asian Australasian Association of Animal Productio 2020 Animal Bioscience Vol.33 No.1
Objective: The objective of this study was to isolate proteolytic microorganisms and evaluate their effects on proteolysis in total mixed ration (TMR) silages of soybean curd residue. Methods: TMRs were formulated with soybean curd residue, alfalfa or Leymus chinensis hay, corn meal, soybean meal, a vitamin-mineral supplement, and salt in a ratio of 25.0: 40.0:30.0:4.0:0.5:0.5, respectively, on a basis of dry matter. The microbial proteinases during ensiling were characterized, the dominate strains associated with proteolysis were identified, and their enzymatic characterization were evaluated in alfalfa (A-TMR) and Leymus chinensis (L-TMR) TMR silages containing soybean curd residue. Results: Both A-TMR and L-TMR silages were well preserved, with low pH and high lactic acid concentrations. The aerobic bacteria and yeast counts in both TMR silages decreased to about 10<sup>5</sup> cfu/g fresh matter (FM) and below the detection limit, respectively. The lactic acid bacteria count increased to 10<sup>9</sup> cfu/g FM. The total microbial proteinases activities reached their maximums during the early ensiling stage and then reduced in both TMR silages with fermentation prolonged. Metalloproteinase was the main proteinase when the total proteinases activities reached their maximums, and when ensiling terminated, metallo and serine proteinases played equally important parts in proteolysis in both TMR silages. Strains in the genera Curtobacterium and Paenibacillus were identified as the most dominant proteolytic bacteria in A-TMR and L-TMR, respectively, and both their proteinases were mainly with metalloproteinase characteristics. In the latter ensiling phase, Enterococcus faecium strains became the major sources of proteolytic enzymes in both TMR silages. Their proteinases were mainly of metallo and serine proteinases classes in this experiment. Conclusion: Proteolytic aerobic bacteria were substituted by proteolytic lactic acid bacteria during ensiling, and the microbial serine and metallo proteinases in these strains played leading roles in proteolysis in TMR silages.