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Pentacene as a hole transport material for high performance planar perovskite solar cells
Xiude Yang,Gang Wang,Debei Liu,Yanqing Yao,Guangdong Zhou,Ping Li,Bo Wu,Xi Rao,Qunliang Song 한국물리학회 2018 Current Applied Physics Vol.18 No.10
A cost-effective and efficient organic semiconductor pentacene was developed as a hole transport layer (HTL) material to replace classical PEDOT:PSS for planar perovskite solar cells (PSCs). As expected, the pentacene based device exhibits power conversion efficiency (PCE) of 15.90% (Jsc of 19.44 mA/cm2, Voc of 1.07 V, and FF of 77%), comparable to the PEDOT:PSS based device (PCE of 15.65%, Jsc of 18.78 mA/cm2, Voc of 1.07 V, and FF of 77%) under the same experimental conditions. The excellent performance of vacuum deposited pentacene is mainly attributed to the high efficient charge extraction and transfer in device due to the high-quality perovskite film grown on the top of pentacene substrate and a favorable energy-level alignment together with a desired downward band bending formed at the perovskite/pentacene interface. Our research has confirmed that pentacene could be served as a promising HTL material to achieve effective and potentially economical planar type PSCs.
Yang Xiude,Li Ping,Wu Bo,Li Hongwei,Zhou Guangdong 한국물리학회 2021 Current Applied Physics Vol.32 No.-
For achieving more effective mechanical energy conversion, based on low-cost and flexible polydimethylsiloxane (PDMS) and polyvinylidene fluoride (PVDF) polymer film as triboelectric and piezoelectric function layer respectively, a polymer-based hybrid piezoelectric-triboelectric nanogenerator (PT-NG) with a structure of Al/ PVDF/Cu-PDMS/indium tin oxide (ITO)/polyethylene terephthalate (PET) has been demonstrated. The device has realized the simultaneous triboelectric and piezoelectric conversions in one structure. In addition, when PDMS and PVDF are further modified by graphene quantum dot (GQD) and titanium dioxide (TiO2) nanoparticles respectively, both triboelectric and piezoelectric outputs of the modified device are greatly enhanced synchronously. The experimental results have indicated that the increase of triboelectric output is due to the improvement of dielectric properties of PDMS film doped with conductive GQDs as well as the enhancement of the effective contact caused by the change of PDMS surface microstructure. While the promotion of piezoelectric output is mainly attributed to the fact that PVDF film after TiO2 modification induces more polarized β phase with a polarization-free process. Accordingly, the modified device converts mechanical energy into electricity more effectively, which shows a promising prospect in the fields of flexibility display, electronic skin, wearable electronic products and self-powered sensors.
Xiude Yang,Debei Liu,Ping Li,Bo Wu,Haishen Huang,Tingyan Zhou,Guangdong Zhou 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2018 NANO Vol.13 No.09
By adopting N, N-Dimethylformamide (DMF) atmosphere annealing at room temperature, planar perovskite solar cells with a p-i-n structure of ITO/PEDOT:PSS/Perovskite/PCBM/C60/Al are fabricated by a simple one-step solution process in ambient air with humidity around 50%, and the influence of DMF atmosphere on perovskite solar cells (PSCs) is systematically investigated. Compared to the reference device without DMF reaction, the perovskite films treated by modest DMF annealing show a better distribution and a higher densification, and thus the power conversion efficiency (PCE), short circuit current density (Jsc) and fill factor (FF) are increased by about 17%, 8% and 6%, respectively. This work displays the importance of solvent annealing for perovskite film prepared by the one-step spin-coating method, and possibly provides a simple and cost-effective way to efficiently fabricate PSCs in ambient air.
Guo, Qingjie,Liu, Yongzhuo,Jia, Weihua,Yang, Mingming,Hu, Xiude,Ryu, Ho-Jung American Chemical Society 2014 ENERGY AND FUELS Vol.28 No.11
<P>Chemical looping combustion (CLC) of coal is an attractive technology with inherent CO<SUB>2</SUB> separation and high energy utilization efficiency. The large-scale preparation of a cheap oxygen carrier with high attrition resistance challenges the scale-up step of CLC reactor systems. To improve the reactivity between the CaSO<SUB>4</SUB>/bentonite (CaBen) oxygen carrier and coal, CaSO<SUB>4</SUB>–Fe<SUB>2</SUB>O<SUB>3</SUB>/bentonite (CaFeBen) and CaSO<SUB>4</SUB>–K<SUB>2</SUB>CO<SUB>3</SUB>/bentonite (CaKBen), decorated by Fe<SUB>2</SUB>O<SUB>3</SUB> and K<SUB>2</SUB>CO<SUB>3</SUB>, respectively, were prepared in this work. The active component content, multi-cycle reactivity, and enhancement mechanism of two decorated oxygen carriers were investigated in a fluidized bed with steam as the gasification–fluidization medium. Finally, three types of coals, including lignite, bitumite, and anthracite, were used as fuel. The addition of Fe<SUB>2</SUB>O<SUB>3</SUB> and K<SUB>2</SUB>CO<SUB>3</SUB> can improve the reactivity of the CaBen oxygen carrier but degrade the attrition resistance slightly. The multiple-cycle experiments indicated that Fe<SUB>2</SUB>O<SUB>3</SUB> itself is the oxygen carrier for coal CLC with high reactivity, while K<SUB>2</SUB>CO<SUB>3</SUB> acts as the catalysis for coal gasification. The carbon conversion rate of the three coals that reacted with the CaKBen oxygen carrier was higher than that with CaFeBen as the oxygen carrier because of catalysis of potassium on the coal gasification reaction. However, the CaKBen oxygen carrier particles were seriously sintered, and the potassium content in the oxygen carrier reduced with the increasing redox cycles. The coals with high volatile and ash contents have a high instantaneous rate of carbon conversion reacted with two decorated oxygen carriers.</P>
RNA-seq for comparative transcript profiling in leaves of strawberry seedlings under salinity stress
Zhang Rui,Du Qiuli,Zhao Wenzhe,Yang Long,Li Dong-mei,Chen Xiude,Xiao Wei,Fu Xiling,Yang Chao,Li Ling 한국식물생명공학회 2023 Plant biotechnology reports Vol.17 No.1
As a major economic crop, strawberry (Fragaria × ananassa Duch.) has been widely planted in the world because of their adaptability and high economic efficiency. In the process of strawberry production, the traditional techniques of furrow irrigation, irrigating irrigation and water and fertilizer management are still relatively common, resulting in secondary salinization of the soil and an imbalance of nutrient ratio, resulting in a decrease in strawberry yield and quality. A total of 2334, 2718 differentially expressed genes (DEGs) were identified in the 3-day, 6-day salt-treated leaf tissues compared with the controls, respectively. Based on the analysis of DEG function annotation and enrichment, a pattern of strawberry leaves response to NaCl stress was proposed. The processes related to plant hormone signal and lipid metabolism pathway were noted in the response of strawberry leaves to NaCl. Our transcriptome data provides valuable insights into genes involved in the growing process of strawberry seedlings under salt stress, and may help in developing seedlings with enhanced responses to salt stress in the years to come.