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Promotional effect of Ce in NH3-SCO and NH3-SCR reactions over Cu-Ce/ SCR catalysts
Wenjie Liu,Yifei Long,Shinian Liu,Yongyan Zhou,XinTong,Yajie Yin,Xiaoyi Li,Kang Hu,Jiangjun Hu 한국공업화학회 2022 Journal of Industrial and Engineering Chemistry Vol.107 No.-
Commercial V-W-Ti catalysts were modified with Cu and different contents of Ce to remove slip ammoniaand remaining nitrogen oxide from the end stage of SCR technology. The activities of NH3 oxidation byO2 (NH3-SCO) and NO reduction by NH3 (NH3-SCR) of these catalysts were examined from 150 to 400 ℃. The consequences indicated that the addition of Ce and Cu could considerably enhance NH3 oxidation andNO reduction capacity of the catalysts and Ce was conducive to reduce the detrimental effects of H2O andSO2. The characterization tests indicated that the surface active oxygen increased because of the interactionbetween V, Cu and Ce. Moreover, the loaded Ce and Cu contributed to enhance the surface acidityand redox property of SCR catalysts.