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RISS 인기검색어
- 검색키워드
- 저자 : Hou Chenxi (검색결과 5 건)
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Ultrasonic-assisted dissolution of U3O8 in carbonate medium
Hou Chenxi,He Mingjian,Fang Haofan,Zhang Meng,Gao Yang,Jiao Caishan,He Hui 한국원자력학회 2023 Nuclear Engineering and Technology Vol.55 No.1
Ultrasound-assisted dissolution of U3O8 powder in carbonate solution was explored to determine if and how ultrasound act during the dissolution. The variation of U3O8 solid particles and uranyl complexes under ultrasound treatment and magnetic stirring was observed in carbonate media. The results show that the use of ultrasound can increase the solubility and dissolution rate of U3O8 powder than that under magnetic stirring. The crush of U3O8 particles and the reduction of the activation energy (Ea, kJ/ mol) of U3O8 dissolution reaction were observed, which both play an important role in the ultrasonicassisted dissolution of U3O8 in carbonate-peroxide solution. Meanwhile, there is no observation of the ultrasound effect on the distribution of uranyl species and hydrolysis of uranyl complexes during the ultrasound treatment in carbonate-peroxide solution. Although the generation of $OH radicals under ultrasound (22 ± 2 kHz) was observed, the oxidation of $OH had little effect on the dissolution of U3O8 in the carbonate-peroxide solution system.
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Development of a Novel 30 kV Solid-state Switch for Damped Oscillating Voltage Testing System
Hou, Zhe,Li, Hongjie,Li, Jing,Ji, Shengchang,Huang, Chenxi The Korean Institute of Power Electronics 2016 JOURNAL OF POWER ELECTRONICS Vol.16 No.2
This paper describes the design and development of a novel semiconductor-based solid-state switch for damped oscillating voltage test system. The proposed switch is configured as two identical series-connected switch stacks, each of which comprising 10 series-connected IGBT function units. Each unit consists of one IGBT, a gate driver, and an auxiliary voltage sharing circuit. A single switch stack can block 20 kV-rated high voltage, and two stacks in series are proven applicable to 30 kV-rated high voltage. The turn-on speed of the switch is approximately 250 ns. A flyback topology-based power supply system with a front-end power factor correction is built for the drive circuit by loosely inductively coupling each unit with a ferrite core to the primary side of a power generator to obtain the advantages of galvanic isolation and compact size. After the simulation, measurement, and estimation of the parasitic effect on the gate driver, a prototype is assembled and tested under different operating regimes. Experimental results are presented to demonstrate the performance of the developed prototype.
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Development of a Novel 30 kV Solid-state Switch for Damped Oscillating Voltage Testing System
Zhe Hou,Hongjie Li,Jing Li,Shengchang Ji,Chenxi Huang 전력전자학회 2016 JOURNAL OF POWER ELECTRONICS Vol.16 No.2
This paper describes the design and development of a novel semiconductor-based solid-state switch for damped oscillating voltage test system. The proposed switch is configured as two identical series-connected switch stacks, each of which comprising 10 series-connected IGBT function units. Each unit consists of one IGBT, a gate driver, and an auxiliary voltage sharing circuit. A single switch stack can block 20 kV-rated high voltage, and two stacks in series are proven applicable to 30 kV-rated high voltage. The turn-on speed of the switch is approximately 250 ns. A flyback topology-based power supply system with a front-end power factor correction is built for the drive circuit by loosely inductively coupling each unit with a ferrite core to the primary side of a power generator to obtain the advantages of galvanic isolation and compact size. After the simulation, measurement, and estimation of the parasitic effect on the gate driver, a prototype is assembled and tested under different operating regimes. Experimental results are presented to demonstrate the performance of the developed prototype.
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Preparation of self‑supporting Co3S4/ S‑rGO film catalyst for efficient oxygen evolution reaction
Liang Chen,Liying Hu,Chenxi Xu,Lanyun Yang,Wei Wang,Junlin Huang,Minjie Zhou,Zhaohui Hou 한국탄소학회 2023 Carbon Letters Vol.33 No.7
Exploring cheap and efficient oxygen evolution reaction (OER) catalysts is extremely vital for the commercial application of advanced energy storage and conversion systems. Herein, a self-supporting Co3S4/ S-doped reduced graphene oxide ( Co3S4/S-rGO) film catalyst is successfully prepared by a blade coating coupled with high-temperature annealing strategy, and its morphology, structure and composition are measured and analyzed. It is substantiated that the as-synthesized Co3S4/ S-rGO film possesses unique self-supporting structure, and is composed of uniformly dispersed Co3S4 nanoparticles and highly conductive S-rGO, which benefit the exposure of catalytic sites and electron transfer. By reason of the synergistic effect of the two individual components, the self-supporting Co3S4/ S-rGO film catalyst displays outstanding catalytic performance towards OER. As a consequence, the Co3S4/ S-rGO film catalyst delivers an overpotential of 341 mV at 10 mA cm-2, and the current attenuation rate is only 2.6% after continuous operation for 4 h, verifying excellent catalytic activity and durability. Clearly, our results offers a good example for the construction of high-performance self-supporting carbon-based composite film catalysts for critical electrocatalytic reactions.
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Chen Liang,Yang Lanyun,Xu Chenxi,Chen Kechun,Wang Wei,Yang Liming,Hou Zhaohui 한국탄소학회 2023 Carbon Letters Vol.33 No.2
Recently, hollow carbon spheres (HCS) have aroused great interests in the field of energy storage and conversion owing to their unique morphology, structure and other charming properties. Nevertheless, unsatisfactory electrical conductivity and relatively poor volumetric energy density caused by inevitable gaps between discrete carbon spheres greatly impede the practical application of HCS. In this work, for the first time we propose a novel dual-template strategy and successfully fabricate interconnected 3D hollow N-doped carbon network (HNCN) by a facile and scalable pyrolysis process. By systematical characterization and analysis, it can be found that HNCN is assembled by HCS and lots of mesoporous carbon. Compared to the counterparts, the obtained HNCN exhibits unique 3D interconnected architecture, larger specific surface area, hierarchical meso/macropore structure, higher structure defects, higher N doping amount and more optimized N configurations (especially for pyridinic-N and graphitic-N). As a result, these advantageous features endow HNCN with remarkably promoted electrochemical performance for supercapacitor and oxygen reduction reaction. Clearly, our proposed dual-template strategy provides a good guidance on overcoming the intrinsic shortcomings of HCS, which undoubtedly broadens their application in energy storage and conversion.
ScienceON
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