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- 저자 : He Yiting (검색결과 2 건)
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Ying Cao,Aoqi Zhu,Jianmin He,Jianhua Wu,Mingjin Xue,Yiting Xu,Birong Zeng,Guorong Chen,Lizong Dai 한국공업화학회 2022 Journal of Industrial and Engineering Chemistry Vol.115 No.-
A novel kind of core cross-linked assemblies formed from a ‘‘semi-amphiphilic” block copolymer, poly(syringaldehyde methacrylate)-block-poly (dopamine methacrylate-co-methyl methacrylate-costyrene)(PSMA-b-P(DMA-co-MMA-co-St)), was designed and served as the carrier for anti-corrosiveand corrosion detective molecules. Different from the core cross-linked micelles formed by the amphiphilicpolymers in water, the core cross-linked assemblies in this research were formed from the ‘‘semiamphiphilic”block copolymer, which took advantage of the different compatibility between epoxy andthe blocks in the polymer, leading to the self-assembly behavior happening in the organic resin, whilethey shared the advantages of traditional core cross-linked micelles with the properties of being stable,stimuli-responsive and multifunctional. The pH-responsive properties of the assemblies and their complexationwith Fe3+ caused by the corrosion of the steel were confirmed by UV spectrophotometry andXPS analysis of the corrosive products. The controlled release of corrosion inhibitors was fully reflectedby the expansion of the capacitor ring and the increase of the coating resistance (Rc) with the extensionof the immersion time, which was got via fitting the electrochemical impedance spectroscopy (EIS) datawith the equivalent electric circuits. Ultimately, the anti-corrosive mechanism of smart coating with thefunctional core cross-linked assemblies were also illustrated.
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Yan Rui,Wang Kai,Tian Xiaodong,Li Xiao,Yang Tao,Xu Xiaotong,He Yiting,Lei Shiwen,Song Yan 한국탄소학회 2020 Carbon Letters Vol.30 No.3
Heteroatoms in situ-doped hierarchical porous hollow-activated carbons (HPHACs) have been prepared innovatively by pyrolyzation of setaria viridis combined with alkaline activation for the frst time. The micro-morphology, pore structure, chemical compositions, and electrochemical properties are researched in detail. The obtained HPHACs are served as outstand�ing electrode materials in electrochemical energy storage ascribe to the particular hierarchical porous and hollow structure, and the precursor setaria viridis is advantage of eco-friendly as well as cost-efective. Electrochemical measurement results of the HPHACs electrodes exhibit not only high specifc capacitance of 350 F g−1 at 0.2 A g−1, and impressive surface specifc capacitance (Cs) of 49.9 μF cm−2, but also substantial rate capability of 68% retention (238 F g−1 at 10 A g−1) and good cycle stability with 99% retention over 5000 cycles at 5 A g−1 in 6 M KOH. Besides, the symmetrical supercapacitor device based on the HPHACs electrodes exhibits excellent energy density of 49.5 Wh kg−1 at power density of 175 W kg−1 , but still maintains favorable energy density of 32.0 Wh kg−1 at current density of 1 A g−1 in 1-ethy-3-methylimidazolium tetrafuoroborate (EMIMBF4) ionic liquid electrolyte, and the excellent cycle stability behaviour shows the nearly 97% ratio capacitance retention of the initial capacitance after 10,000 cycles at current density of 2 A g−1. Overall, the results indicate that HPHACs derived from setaria viridis have appealing electrochemical performances thus are promising electrode materi�als for supercapacitor devices and large-scale applications.
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