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Badrut Tamam Ibnu Ali,Cininta Nareswari,Triyanda Gunawan,Nurul Widiastuti,Yuly Kusumawati,Juhana Jaafar,Hens Saputra,Dety Oktavia Sulistiono 한국공업화학회 2023 Journal of Industrial and Engineering Chemistry Vol.127 No.-
Polyethylene terephthalate (PET) is a widely used polymer in packaging products, leading to the daily disposalof millions of PET bottles as waste. 1.1 to 8.8 million tonnes of plastic waste enter the sea each year. The environmental challenge of non-biodegradable PET waste can be addressed by utilizing it as a thinlayermembrane for gas separation. This study modified the PET membrane by blending it with Pebaxpolymer and adding zeolite as a filler to enhance its performance. Characterization techniques, includingFTIR, SEM, TGA, tensile strength testing, and contact angle measurements, were performed on all modifiedmembranes. The membranes were prepared using phase inversion via immersion precipitation. Theresults showed that the PET waste membrane had a denser surface pore morphology and asymmetricalcross-sectional pores than other membranes. Adding Pebax and zeolite resulted in a more regularsponge-like pore structure. The PET, PET-Pebax, and PET-Zeolite NaY-Pebax membranes exhibited hydrophilicproperties, as indicated by contact angle values ranging from 48-78. Regarding CO2/CH4 separation,the 9% PET-Pebax membrane had the highest CO2 permeability, a 21% increase from the originalPET waste membrane. Adding zeolite to the 9% PET-Pebax membrane increased CO2 permeability to1044%.