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Eu3+-site occupation in CaTiO3 perovskite material at low temperature
Fengfeng Chi,Yanguang Qin,Shaoshuai Zhou,Xiantao Wei,Yonghu Chen,Changkui Duan,Min Yin 한국물리학회 2017 Current Applied Physics Vol.17 No.1
In order to clarify the site occupancy of rare-earth ions in rare-earth doped perovskite materials, the undoped pure CaTiO3 and Eu3þ-doped CaTiO3 samples with a series of Ca/Ti ratio were synthesized via high-temperature solid-state reaction method. X-ray diffraction (XRD) powder patterns confirm that the crystal structure keeps invariant at various Ca/Ti ratios. Measurement results of unit-cell parameters and X-ray photoelectron spectroscopy (XPS) indicate that Eu3þ ions enter into the Ca2þ site. The highresolution photoluminescence spectra of Eu3þ ions at 20 K in all samples did not witness a significant change under the excitation at different wavelength, implying that Eu3þ ions occupy only one type of site. Considering the small spectral splitting range of 5D0/7F2 transition and the large intensity ratio of 5D0 / 7F2/5D0 / 7F1, it can be concluded that Eu3þ occupies Ca2þ site with larger coordinate numbers rather than Ti4þ site.
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A new red-emitting phosphor of Eu3+-doped Sr2MgMoxW1−xO6 for solid state lighting
Shuo Li,Xiantao Wei,Kaimo Deng,Xiuna Tian,Yanguang Qin,Yonghu Chen,Min Yin 한국물리학회 2013 Current Applied Physics Vol.13 No.7
The white light-emitting diode has recently attracted great attention as a promising candidate for next generation lighting. The solid solution of Sr1.80Eu0.10Li0.10MgMoxW1-xO6 was synthesized via hightemperature solid-state reaction and this solid solution is treated as a promising red emitting phosphor for white light-emitting diodes. In our cases, the X-ray diffraction, excitation spectra, emission spectra and decay curves of these solid solutions were measured as a function of the Mo/W ratio to characterize the structural and luminescent properties. The excitation bands of the series of phosphors are consistent well with the region of near ultraviolet light, and the phosphors present better color purity than the commercial phosphor Y2O2S:Eu3þ in current use. Taking these properties into consideration,this kind of material may find a great potential application as a red phosphor for near-ultraviolet excited white light-emitting diodes.
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