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Phase Diagram and Transport Properties of Y1−xNdxCo2 Pseudo-binary Alloys
A. T. Burkov,M. Takeda,A. Teruya,S. Watanabe,Y. Hiranaka,A. Nakamura,M. Hedo,T. Nakama,K. Yagasaki,Y. Takaesu,K. Uchima,Y. Uwatoko 한국물리학회 2013 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.62 No.12
The electrical resistivity and the thermopower S of pseudo-binary Y1−xNdxCo2 alloys have beenmeasured at temperatures from 2 to 300 K under pressures up to 3.5 GPa. NdCo2 is a ferromagnetwith a Curie temperature TC of 98 K. In the ferromagnetic phase, it undergoes a 4f spin-reorientationtransition at TR = 40 K. At this transition, the easy direction of 4f magnetization is changed from[100] at temperatures above TR to [110] below TR. The system phase diagram TC(x, P) and TR(x, P)is inferred from the temperature dependencies of the electrical resistivity and the thermopower. The Curie temperature of the alloys, TC decreases with decreasing Nd concentration x and vanishesaround xc = 0.3. Above xc, the Curie temperature decreases with increasing pressure. The spinreorientationtemperature weakly depends on the composition and on the pressure until it mergeswith TC. There is a large region of the phase diagram, partly overlapping with the ferromagneticphase, where the cobalt 3d electron system is non-uniformly magnetized due to spatial fluctuationsof the 4f-3d exchange field related to a random distribution of Nd 4f magnetic moments over the Rsublattice. In this region, large static 3d magnetic fluctuations govern the electronic transport.
T. Sakurai,K. Fujimoto,S. Okubo,H. Ohta,Y. Uwatoko 한국자기학회 2013 Journal of Magnetics Vol.18 No.2
We have developed a high-field and high-frequency ESR system using a commercially available magnetometer equipped with the superconducting quantum interference device (SQUID). This is magnetization detection type ESR and ESR is observed as a change of the magnetization at the resonance condition under irradiation of the electromagnetic wave. The frequency range is from 70 to 315 GHz and the maximum magnetic field is 5 T. The sensitivity is estimated to be 10<SUP>13</SUP> spins/G. The advantage of this system is that the high-field ESR measurements can be made very easily and quantitatively. Moreover, this high-field ESR can be applied to the measurements under pressure by using a widely used piston-cylinder pressure cell.