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Excitation Energy Transfer in Organic Materials: From Fundamentals to Optoelectronic Devices
Laquai, Fré,dé,ric,Park, Young-Seo,Kim, Jang-Joo,Basché,, Thomas WILEY-VCH Verlag 2009 Macromolecular Rapid Communications Vol.30 No.14
<P>In this review, we discuss investigations of electronic excitation energy transfer in conjugated organic materials at the bulk and single molecule level and applications of energy transfer in fluorescent and phosphorescent organic light emitting devices. A brief overview of common descriptions of energy transfer mechanisms is given followed by a discussion of some basic photophysics of conjugated materials including the generation of excited states and their subsequent decay through various channels. In particular, various examples of bimolecular excited state annihilation processes are presented. Energy transfer studies at the single molecule level provide a new tool to study electronic couplings in simple donor/acceptor dyads and conjugated polymers. Finally, energy transfer in organic electronic devices is discussed with particular emphasis on triplet emitter doped OLEDs and blends for white light emission.</P><P> <img src='wiley_img/10221336-2009-30-14-MARC200900309-gra001.gif' alt='wiley_img/10221336-2009-30-14-MARC200900309-gra001'> </P> <B>Graphic Abstract</B> <P>Understanding energy transfer in small organic molecules and conjugated polymers is a prerequisite for the design of novel materials for organic optoelectronics. Bulk as well as single molecule studies of energy transfer yield information which ultimately will help to optimize device structures. <img src='wiley_img/10221336-2009-30-14-MARC200900309-content.gif' alt='wiley_img/10221336-2009-30-14-MARC200900309-content'> </P>