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A FULL CHARGE SEPARATION OVER THE TWO SAME CHROMOPHORES IN A PHOTOSYNTHETIC TETRAD
Osuka, Atsuhiro,Marumo, Shinji,Okada, Tadashi,Taniguchi, Seiji,Mataga, Noboru,Ohno, Takeshi,Nozaki, Koichi,Yamazaki, Iwao,Nishimura, Yoshinobu Korean Society of Photoscience 1997 Journal of Photosciences Vol.4 No.3
The synthesis and excited-state dynamics are described for a tetrad (ZC - ZP - ZP - I) consisting of zinc chlorin (ZC), zinc porphyrin (ZP), zinc porphyrin (ZP), and pyromellitimide (I), which upon photoexcitation provides a fully charge-separated state (ZC$^+$- P - ZP - l$^- $) with lifetimes of 230 $\mu$s in THF and > 50$ \mu$s in DMF at room temperature via a stepwise electron-transfer relay that has been detected by the ps-time resolved transient absorption spectroscopy.