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Polaron Localization at Interfaces in High-Mobility Microcrystalline Conjugated Polymers
Zhao, N.,Noh, Y.-Y.,Chang, J.-F.,Heeney, M.,McCulloch, I.,Sirringhaus, H. WILEY-VCH Verlag 2009 ADVANCED MATERIALS Vol.21 No.37
<B>Graphic Abstract</B> <P>The charge-induced optical absorptions of two-dimensional polarons in semicrystalline, high-mobility conjugated polymers are investigated as a function of distance from an interface with polymer gate dielectrics of different dielectric constants. For high-k dielectrics, polarons in the accumulation layer at the interface are found to be more localized than those in the bulk. <img src='wiley_img/09359648-2009-21-37-ADMA200900326-content.gif' alt='wiley_img/09359648-2009-21-37-ADMA200900326-content'> </P>