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Rational design of a phthalocyanine–perylenediimide dyad with a long-lived charge-separated state
Blas-Ferrando, Vicente M.,Ortiz, Javier,Bouissane, Latifa,Ohkubo, Kei,Fukuzumi, Shunichi,Ferná,ndez-Lá,zaro, Fernando,Sastre-Santos, Á,ngela The Royal Society of Chemistry 2012 Chemical communications Vol.48 No.50
<P>A new ZnPc–PDI dyad presenting for the first time a charge-separated state lower in energy than the triplet excited state of the ZnPc and PDI has been synthesized. The rational design implies the substitution of the ZnPc with phenoxy groups and the bay substitution of the PDI with sulfonyl substituents. The lifetime of the charge-separated state was 72 μs.</P> <P>Graphic Abstract</P><P>The longest charge-separated state so far, 72 μs, without the addition of external components, for phthalocyanine–perylenediimide arrays has been described. <IMG SRC='http://pubs.rsc.org/services/images/RSCpubs.ePlatform.Service.FreeContent.ImageService.svc/ImageService/image/GA?id=c2cc31087b'> </P>