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Efficiently visible and 2 μm infrared emission in K2YbF5: Ce3+/Ho3+ microcrystals
Hao Dong,Guangping Zhu,Min Zhang,Kai Dai,Qiang Li,Chaopeng Cui 한국물리학회 2020 Current Applied Physics Vol.20 No.6
Ho3+/Ce3+ co-doped K2YbF5 microcrystals were synthesized by solvent-thermal method. Under excitation of 980 nm laser diode, effectively visible and 2 μm-infrared luminescence of Ho3+ ion were obtained in the microcrystals. By changing Ce3+-ion doping concentration, the luminescence properties of visible and 2 μm emission were effectively regulated. At low Ce3+-ion doping level, the red and green upconversion emission obviously increases and decreases respectively with the increase of Ce3+-ion amount in the samples, meanwhile the intensity of 2 μm fluorescence changes very little. At high Ce3+-ion doping level, the intensities of the red and green emission both decrease with the increase of Ce3+-ion concentration, while the 2 μm emission intensity increases obviously. In the sample doped with 16% Ce3+ ion, the intensity of 2 μm emission is about 4.5 times that of the sample without Ce3+ ion, and the corresponding quantum efficiency is about 78.3%. The result is attributed to the influence of the different cross relaxation between Ho3+ and Ce3+ ion in luminescence process at low and high Ce3+-ion doping concentration. The corresponding luminescence mechanism and energy transfer process were discussed in detail.
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Jiaqi Dong,Boxin Wang,Xuexin Yan,Xinchuan Xu,Guangping Xiao,Qingbo Yu,Meng Yao,Qing Wang 대한토목학회 2022 KSCE JOURNAL OF CIVIL ENGINEERING Vol.26 No.5
The rebound index Cr is an important design parameter in engineering construction, and its determination is cumbersome and susceptible to errors. Explaining the macroscopic rebound characteristic parameter Cr from the perspective of microscopic mechanism is an important research area that is addressed in this study. In this paper, the different soil parameters, including the Cr parameter and the physical parameters (void ratio e, liquid limit water contentwL, and plasticity index Ip), have been determined through experiments for the undisturbed clay of Chongming East Shoal (CES), Shanghai. Further, scanning electron microscopy (SEM) imaging was used to analyze the microstructural features. Through SEM, the grey correlation degree, the average abundance of structural units ACp and the average equivalent diameter of pores ADv were determined as the soil microstructure parameters with the most significant correlation with Cr. The predictive analysis model of Cr was then carried out combined with the PSO-SVM algorithm. In order to evaluate the influence of microscopic parameters of soil on the prediction accuracy, four sets of input parameter combinations were used. The results indicate the high prediction accuracy of the developed model. Sensitivity analysis was also carried out, which showed that the sensitivity of Cr to ACp and ADv was significantly lower than e; however, the difference from wL and Ip was small, indicating that it is imperative to consider microscopic parameters while predicting Cr. This study, thus, provides a basis and method for predicting the rebound index of soil from the microstructure perspective.
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Experimental and theoretical analysis of element mercury adsorption on Fe3O4/Ag composites
Lu Dong,Jiangkun Xie,Guangping Fan,Yaji Huang,Jun Zhou,Qingke Sun,LiangWang,Zhengwen Guan,Di Jiang,Ye Wang 한국화학공학회 2017 Korean Journal of Chemical Engineering Vol.34 No.11
A novel magnetic nano-sorbent Fe3O4/Ag was synthesized and applied to capture the elemental mercury from the simulated flue gas. The morphology, components and crystal phase of the sorbents were characterized by transmission electron microscope (TEM), energy dispersive spectrometry (EDS) and X-ray diffraction (XRD), respectively. The mercury removal performance of the sorbents was investigated through the fixed-bed tests. The results indicated that silver was successfully loaded on the surface of Fe3O4 particles, which could significantly enhance the Hg0 removal performance of the sorbents. Flue gas components, including CO2, SO2, and NO, have little impact on the Hg0 removal performance of Fe3O4/Ag sorbents, while O2 has a slightly positive effect. The Hg0 removal efficiency decreased with the increasing of temperature, Hg0 inlet concentration and gas hourly space velocity. Only one broad mercury desorption peak at approximately 210 oC could be observed during the temperature-programmed desorption (TPD) process, which indicated that mercury species existing on the surface of Fe3O4/Ag sorbents might be elemental mercury instead of oxidized mercury. Furthermore, the reusability tests showed that the Fe3O4/Ag sorbents could be efficiently regenerated and reused. Finally, the theoretical analysis based on the DFT method showed that a weak chemisorption of Hg0 on Fe3O4 sorbents changed to a strong chemisorption when silver was loaded. The results of theoretical analysis conformed to the experiments results well.
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Li Xiaojuan,Dong Guangping,Fang Jianmin,Liu Hongjian,Guo Wanlin,Yin Huayang 한국곤충학회 2020 Entomological Research Vol.50 No.7
Dastarcus helophoroides (Fairmaire) (Coleoptera: Bothrideridae) is an effective ectoparasitoid of pine sawyer beetle Monochamus alternatus Hope (Coleoptera: Cerambycidae) which is the major median insect for transmission of pine wood nematode, Bursaphelenchus xylophilus (Steiner et Buhrer) Nickle (Aphelenchida: Parasitaphelenchidae). A sensitive and acute olfactory system is extremely essential for newly hatched larva of D. helophoroides to forage for a host. Therefore, we established the transcriptome of newly hatched D. helophoroides larvae and characterized the expression profiles of olfactory genes. We identified 20 transcripts encoding putative odorant binding proteins (OBPs), 11 putative chemosensory proteins (CSPs), 9 putative odorant receptors (ORs), 11 putative ionotropic receptors (IRs), 7 putative gustatory receptors (GRs) and 4 putative sensory neuron membrane proteins (SNMPs) olfactory genes from the transcriptome of newly hatched D. helophoroides larvae. According to the phylogenetic analysis, 3 OBPs (DhelOBP6, DhelOBP14 and DhelOBP19), 1 CSP (DhelCSP11), 1 OR (DhelOrco1), 3 IRs (DhelIR3, DhelIR6 and DhelIR8), 3 GRs (DhelGR2, DhelGR4 and DhelGR5) and 2 SNMPs (DhelSNMP1 and DhelSNMP3) had high similarities with reported Coleopteran species. The highest expressed olfactory gene was DhelCSP3, followed by DhelOBP8 and DhelCSP2. The expression levels of the majority of OR, IR, GR and SNMP genes were low. These results indicate that CSPs and OBPs may play important roles in the olfactory recognition process in newly hatched D. helophoroides larvae. The findings from the present study are helpful in unraveling the profound mystery between D. helophoroides and M. alternatus, as well as improving the parasitism efficiency of D. helophoroides larvae.
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