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RISS 인기검색어
- 검색키워드
- 저자 : Shojiro Kimura (검색결과 4 건)
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High-field Multi-frequency ESR in the S=2 Heisenberg Antiferromagnetic Chain Compound MnCl3(bpy)
Masayuki Hagiwara,Masami Ikeda,Yuichi Idutsu,Shojiro Kimura,Zentaro Honda 한국물리학회 2013 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.62 No.12
We report the results of high-field multi-frequency electron spin resonance (ESR) experimentson a powder sample of MnCl3 (bpy) (bpy=2, 2’-bipyridine). This compound is one of the rareexamples of the spin (S) 2 quasi one-dimensional (1D) Heisenberg antiferromagnets (HAFs), andmagnetic properties of tiny single crystal samples were reported previously (G. E. Granroth et al.,Phys. Rev. Lett. 77, 1616 (1996).). In our previous paper on this compound (M. Hagiwara et al.,J. Phys.: Conf. Ser. 400, 032014 (2012).), we reported, for the S=2 1D HAF, good agreementbetween experiment and calculation for the temperature dependence of magnetic susceptibility andthe high-field magnetization process at 1.3 K. In this work, we have observed some high-frequencyresonance modes with zero-field gaps of about 800 GHz that may correspond to antiferromagneticresonance modes with orthorhombic anisotropy in a long-range-ordered phase that emerged at lowtemperatures above the critical field at which the energy gap (Haldane gap) closes. The single-ionanisotropy constant D evaluated from the analysis of these ESR modes is larger than that reportedpreviously.
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Multi-step Metamagnetic Processes of PrPd2Si2 Single Crystal
Toru Shigeoka,Tetsuya Fujiwara,Keiichi Koyama,Shojiro Kimura,Kazuo Watanabe 한국물리학회 2013 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.63 No.3
Magnetic studies were performed on PrPd2Si2 single crystals which crystallize in the tetragonalThCr2Si2-type structure. The temperature dependence of the magnetic susceptibility indicates thatthe compound orders antiferromagnetically at temperatures below TN = 3.2 K. The transition wasconfirmed by specific heat measurements. Magnetization measurements at fields up to 18 T showthat the easy magnetization direction is the [100] direction in the basal plane. In the magnetizationprocess, five or four metamagnetic transitions appear; the process is a five (four)-step metamagneticone. The [110] magnetization process is a three-step one. A strong magnetic anisotropy betweenthe [100] and [110] directions is observed within the basal plane for high magnetic fields. Alongthe hard magnetization direction of the c-axis, a metamagnetic transition appears. The B[100] − Tphase diagram was constructed. A magnetic anisotropy between the [100] and [001] directions isalso strong. These behaviors are discussed based on an analysis of crystalline field effects.
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Antiferromagnetic Transition in Ru2CrSi in Magnetic Fields
Masahiko Hiroi,Kaori Uchida,Iduru Shigeta,Masakazu Ito,Keiichi Koyama,Shojiro Kimura,Kazuo Watanabe 한국물리학회 2013 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.62 No.12
In the Heusler compound Ru2CrSi, an antiferromagnetic transition at TN =14 K was revealed byspecific heat and magnetization measurements. In this study the electrical resistivity is measured inmagnetic fields up to 14.5 T, and the antiferromagnetic transition in magnetic fields is investigated. In the temperature dependence of the resistivity at zero field, a clear dip at 15 K and a humpwith a maximum at 9 K are observed. This dip is considered to be due to the antiferromagnetictransition. With increasing magnetic field, the magnitude of the resistivity slightly increases aroundTN; i.e., a positive magnetoresistance is observed. The temperature dependence of the resistivityis hardly affected by increasing the magnetic field. The transition temperature decreases only by 0.3 K even with applying 14.5 T. These results demonstrate that the antiferromagnetic state inRu2CrSi is unusually unaffected by a strong magnetic field.
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Successive Magnetic Transitions of PrRh2 Single Crystals
Yu Okawara,Jingwei Cui,Tetsuya Fujiwara,Toru Shigeoka,Kazuyuki Matsubayashi,Yoshiya Uwatoko,Shojiro Kimura,Kazuo Watanabe 한국물리학회 2013 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.63 No.3
Measurements of the magnetization and the specific heat were performed on a PrRh2 single crystal. A strong magnetic anisotropy with the easy magnetization direction of the c-axis is observed. Four anomalies appear in the temperature dependence of magnetic susceptibility along the c-axis;a cusp at TN=52 K, a high peak at T3=38 K, a shoulder at T2=33 K and a small peak at T1=4K are observed, indicating magnetic transitions. The specific heat also shows four anomalies atthe temperatures where the magnetic anomalies appear, confirming the occurrence of successivemagnetic transitions. A clear two-step metamagnetic process appears along the easy magnetizationdirection of the c-axis at low temperatures. The magnetization in the first step is almost constantand is corresponds to (1/5) Ms (Ms: saturation magnetization), indicating that this field-inducedphase has a long period and a stable magnetic structure. A metamagnetic process is hypothesizedon the basis of the magnetic structure. The B001 − T phase diagram is constructed.
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