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Nobuo Sugimoto,Yukari Hara,Atsushi Shimizu,Tomoaki Nishizawa,Ichiro Matsui,Masataka Nishikawa 한국기상학회 2013 Asia-Pacific Journal of Atmospheric Sciences Vol.49 No.1
The Asian dust events in 2008 (May 24-June 4 in 2008)and in 2009 (March 12-25, October 13-26, and December 15-28 in 2009) were analyzed with the lidar network observations, surface observations in China, Korea, Japan, and Mongolia, and with the chemical transport model CFORS. Transport of Asian dust and mixing of dust with air pollution aerosols were studied. The event of May 24 to June 4 in 2008 was a significant event unusually late in the spring dust season. The dust event of March 12-25, 2009 was an interesting example of elevated dust layer, and transport of dust from the elevated dust layer to the ground by the boundary layer activity was observed with the lidars and surface observations in Japan. The concentration of air pollution aerosols was relatively high during the dust event, and the results suggest that vertical structure as well as transport path is important for the mixing of dust and air pollution aerosols. The dust events in October and December 2009 were examples of dust events in autumn and winter. The online mode CFORS reproduced the observation data generally well, except for the event of May 24 to June 4 in 2008. The results of the fourdimensional variational assimilation of the lidar network data reproduced the dust concentration in Korea and Japan reasonably in that event.
Internal Mixing of Pollutants for Submicron Particles Observed during Springtime in Japan
Matsumoto, Jun,Narukawa, Masahiro,Takahashi, Kenshi,Matsumi, Yutaka,Yabushita, Akihiro,Shimizu, Atsushi,Matsui, Ichiro,Sugimoto, Nobuo Korean Society for Atmospheric Environment 2009 Asian Journal of Atmospheric Environment (AJAE) Vol.3 No.1
Internally mixed states of submicron particles during transport from the Asian continent to the Pacific Ocean were analyzed using a single-particle time-offlight mass spectrometer. The observation was conducted at Tsukuba in Japan in the spring of 2005 in order to investigate springtime transport of particles from the continent. The sum of ion intensities of sulfate (${HSO_4}^-$) detected in particles originating from the continental air masses counted for 75% of that in all particles during the observation. By analyzing correlations among compounds, origins and internally mixed states of compounds were estimated. It was found that nitrate was mixed with sulfate-rich particles as the air mass approached Japan. It was confirmed that Asian mineral dust particles played significant roles for transport of continental sulfate to Japan. As a result of analysis on internal mixing of chlorine and nitrate, it was implied that the chlorine loss in fine sea salt particles had already proceeded at Tsukuba. It was characteristic that fluoride ions were significantly detected, coal combustion in the Asian Continent can be an important source of fluorides detected in Japan through the westward transportation of fine particles including fluorides.