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Optical and Magnetic Properties of MBE-Grown Manganese Sulfide Layers
W. Heimbrodt,L. Chen,H.-A. Krug Von Nidda,A. Loidl,P. J. Klar,L. David,K. A. Prior 한국물리학회 2008 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.53 No.5
Metastable zinc-blende MnS layers of various thicknesses from 1:8 nm to 8:6 nm have been grown by molecular beam epitaxy on (100) GaAs between ZnSe cladding layers. We studied the dependences of the optical and the magnetic properties on the layer thickness. On the one hand, the non-exponential decay of the Mn internal transition is found to be faster for thick erlayer,which is a size effect and not caused by the interfaces. On the other hand, the Neel-temperature is not altered with decreasing layer thickness, but the phase-transition-induced shift of the internal Mn transitions is smaller for thinnerMnSlayers. Thisisexplainedbythedominatingin uenceofMn ions at the interface, which possess a reduced number of Mn neighbors. SQUID measurements in a weak external magnetic eld conrm the optical observations in zero field. However, applying a strong magnetic field reveals the metamagnetic character of these zinc-blende MnS layers. An antiferromagnetic-to-erromagnetic phase transitionis found with increasing external field. Metastable zinc-blende MnS layers of various thicknesses from 1:8 nm to 8:6 nm have been grown by molecular beam epitaxy on (100) GaAs between ZnSe cladding layers. We studied the dependences of the optical and the magnetic properties on the layer thickness. On the one hand, the non-exponential decay of the Mn internal transition is found to be faster for thick erlayer,which is a size effect and not caused by the interfaces. On the other hand, the Neel-temperature is not altered with decreasing layer thickness, but the phase-transition-induced shift of the internal Mn transitions is smaller for thinnerMnSlayers. Thisisexplainedbythedominatingin uenceofMn ions at the interface, which possess a reduced number of Mn neighbors. SQUID measurements in a weak external magnetic eld conrm the optical observations in zero field. However, applying a strong magnetic field reveals the metamagnetic character of these zinc-blende MnS layers. An antiferromagnetic-to-erromagnetic phase transitionis found with increasing external field.
Electronic and phonon excitations in α−RuCl3
Reschke, S.,Mayr, F.,Wang, Zhe,Do, Seung-Hwan,Choi, K.-Y.,Loidl, A. American Physical Society 2017 Physical Review B Vol.96 No.16
<P>We report on terahertz (THz), infrared reflectivity, and transmission experiments for wavenumbers from 10 to 8000 cm(-1) (similar to 1meV-1eV) and for temperatures from 5 to 295 K on the Kitaev candidate material alpha-RuCl3. As reported earlier, the compound under investigation passes through a first-order structural phase transition, from a monoclinic high-temperature to a rhombohedral low-temperature phase. The phase transition shows an extreme and unusual hysteretic behavior, which extends from 60 to 166 K. In passing this phase transition, in the complete frequency range investigated, we found a significant reflectance change, which amounts to almost a factor of two. We provide a broadband spectrum of dielectric constant, dielectric loss, and optical conductivity from the THz to the mid-infrared regime and study in detail the phonon response and the low-lying electronic density of states. We provide evidence for the onset of an optical energy gap, which is on the order of 200 meV, in good agreement with the gap derived from measurements of the dc electrical resistivity. Remarkably, the onset of the gap exhibits a strong blue shift on increasing temperatures.</P>
Electron spin resonance in Eu-based iron pnictides
Krug von Nidda, H.-A.,Kraus, S.,Schaile, S.,Dengler, E.,Pascher, N.,Hemmida, M.,Eom, M. J.,Kim, J. S.,Jeevan, H. S.,Gegenwart, P.,Deisenhofer, J.,Loidl, A. American Physical Society 2012 Physical review. B, Condensed matter and materials Vol.86 No.9