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월유광산산(月留鑛山産) 금(金)-은(銀)광물(鑛物)과 광상(鑛床)의 생성환경(生成環境)
이현구,유봉철,정광영,김기현,Lee, Hyun Koo,Yoo, Bong-Cheal,Jeong, Kwang Young,Kim, Kee Hyun 대한자원환경지질학회 1994 자원환경지질 Vol.27 No.6
The Weolyu gold-silver deposits at Hwanggan, Chungcheongbukdo, is of a late Cretaceous $(74.24{\pm}1.63Ma)$ epithermal vein-type, and is hosted in the quartz porphyry of late Cretaceous age. Based on mineral paragenetic sequence interpreted from vein structure and mineral assemblages, three stages mineralization were distinguished. A variety of ore minerals occurs including pyrite, sphalerite, chalcopyrite, galena with small amount of electrum, native silver, argentite, pearceite, sb-pearceite, argyrotite. The gangue minerals are quartz, rutile, calcite, apatite, fluorite and rhodochrocite. Wall-rock alteration such as pyritization, chloritization, sericitization, silicification is observed near the quartz veins. Au-Ag minerals were crystallized at middle and late stage of the two mineralization sequences. Results from the analysis of fluid inclusion and thermodynamic calculation indicate that Au-Ag mineral deposits were formed primarily by cooling and dilution of hydrothermal fluids($165{\sim}313^{\circ}C$, 0.4~2.4wt.% equivalent NaCl) with some degree mixing of meteoric water.
대전지역 상수도 물의 계절변화에 따른 물리화학적 불균질
이현구,이찬희,서호택 대한자원환경지질학회 2000 자원환경지질 Vol.33 No.6
This study was undertaken to provide a drinking water quality on the basis of physicochemical properties. In this study, the 25 samples of supply waters of the Taejon area were sampled twice (February and August in 1999). Hydrochemistry of the supply water belongs to the $Ca^{2+}$-${HCO_3}^{-1}$ type, whereas the supply water was characterized by the relatively significant enrichment of ${Ca}^{2+}$, ${Na}^{2+}$, ${K}^{2+}$, ${Cl}^{2+}$ ions and heavy metals compared to the original water from the Daecheong lake. Generally, the supply water has a mean values for $10.7^{\circ}C$ of temperature, 6.86 of pH, -12 mV of Eh, 88 ${\mu}S$/cm of EC and 70.379 mg/l of TDS in February, whereas the waters of the same sites in August are a slightly high temperature ($26.1^{\circ}C$), TDS (78.069 mg/l) and extremely high EC (442 ${\mu}S$/cm) value. These values are similar with physicochemical properties of the original lake water depending on the seasonal differences. Results of speciation calculation indicate that potentially toxic ions might exist mainly in the forms of free metal (${Cu}^{2+}$ or ${Zn}^{2+}$) and a small amount of ${CO_3}^{2-}$and ${OH}^{-}$in the supply water. The water seemed to be in equilibrium with kaolinite field of the normal stability diagrams for the natural water. Based on enrichment parameter of the supply water normalized by original lake water composition, the average value of those parameter can be calculated with nearly 1.00, but the those values for Cu+Zn possible source of decrepit pipe lines are 126.75 in February and 115.63 in August samples. The parameter values varied with sampling sites, however, do not exceed by chemistry of drinking water standard. Solid compounds remained on the membrane filter papers after filtration are adhered to pale yellow or yellowish brown colored dissolved solids and precipitates, which are coated by 0.02 to 0.35 mm thick per 500 ml with colloidal particles of about 1 to 2${\mu}m$ size. The particles are mainly Fe-Cu-Zn compounds and partly detected to Mn and Pb.
한국(韓國) 장군광산(將軍鑛山)의 황석석(黃錫石)에 대(對)하여 -장군(將軍) 연(鉛)·아연(亞鉛)·은(銀) 광석광물(鑛石鑛物)의 지식(知識)에의 기여(寄與) (3)-
이현구,이마이 나오야,Lee, Hyun Koo,Imai, Naoya 대한자원환경지질학회 1986 자원환경지질 Vol.19 No.no.spc
In the Janggun mine, stannite occurs as anhedral grains, up to 500 micrometer in long dimension, closely associated with sphalerite, chalcopyrite, arsenopyrite, pyrrhotite, galena and rhodochrosite in the periphery of the South ore body. In reflected light, stannite is grayish yellow green in color and exhibits moderate bireflectance and strong anisotropism without any intenal reflections. Reflection; Rmax. =29.0, Rmin. =27.8 percent at a wavelength of 560nm, and VHN; 219~244kg/mm at a 50g load. The chemical composition on the average from 35 spot analyses by electron microprobe is, Cu 28.0, Fe 12.7, Zn 2.9, Mn 0.2, Sn 25.8, S 30.3, sum 99.9 (all in weight percent); the corresponding chemical formula as calculated on the basis of total atoms=8 is, Cu 1.88 Fe 0.97 Zn 0.19 Mn 0.02 Sn 0.93 S 4.01, which fulfills approximately the ideal formula of $Cu_2FeSnS_4$. The strongest reflections on the X-ray diffraction patterns are; $3.10{\AA}$ (10) (112), $2.72{\AA}$ (5) (020, 004), $1.922{\AA}$ (5) (024), $1.642{\AA}$ (3) (132), $1.244{\AA}$ (3) (143, 136, 235), $1.111{\AA}$(3) (244), $0.958{\AA}$ (1) (048, 422), the patterns are identical with those of literature. From the textural evidence of the microscopic observation, the mineral is considered to have been formed at the middle stage of hydrothermal lead-zinc-silver mineralization.
이현구,김상중,김문영,Lee, Hyun Koo,Kim, Sang Jung,Kim, Mun Young 대한자원환경지질학회 1998 자원환경지질 Vol.31 No.1
Copper mineralization of the Donghwa and Hwanghagsan mines was deposited in hydrothermal quartz veins which filled fissures in Cretacous sedimentary rocks. Ore minerals are pyrite, sphalerite, chalcopyrite, bornite, galena, wittichenite and unidentified Cu-Bi-Pb-Sb-S mineral. On the basis of salinities and homogenization temperatures for fluid inclusions, the Donghwa deposit was deposited from $300^{\circ}C$ to $220^{\circ}C$ with 2.5 to 0.2 wt.% eq. NaCl, and the Hwanghagsan deposits was deposited from $300^{\circ}C$ to $160^{\circ}C$ with 4.0 to 0.0 wt.% eq. NaCl. Evidence of boiling suggests pressure of 170 to 60 bar, these pressures correspond to 1700 m to 600 m. The ${\delta}^{34}S_{H_2S}$ values of the Donghwa deposit (4.8~7.4%) are higher than those of the Hwanghagsan deposit (3.5~4.5%), sulfur isotope compositions indicate that ore fluids partially reacted with meteoric water and wall-rock. Equilibrium thermodynamic interpretation indicates that the temperature versus $fs_2$ of the Donghwa deposit (> $420^{\circ}C$, $10^{-3.2}atm$) is higher condition than that of the Hwanghagsan deposit (> $290^{\circ}C$, $10^{-7.0}atm$). K-Ar ages for biotite granite and quartz porphyry in the study area are 64.7 Ma, and 60.9 Ma, reapectively. Mineralization age using sericite in the Donghwa deposits is 59.8 Ma. Therfore, Copper mineralization in the study area was associated with acidic igneous activity such as biotite granite or quartz porphyry.