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M¨ossbauer Spectroscopy of Fe-doped Valence-fluctuating α-YbAlB4
Yui Sakaguchi,Shugo Ikeda,Hisao Kobayashi,Kentaro Kuga,Keita Sone,Satoru Nakatsuji 한국물리학회 2013 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.62 No.12
The magnetic properties of high-quality 25 at.% Fe doped α-YbAlB4 with an orthorhombicPbam structure were investigated by using magnetization measurements and 57Fe M¨ossbauer spectroscopy. The temperature dependence of the magnetization along the a-axis showed anomaliesat TN2 7.7 K and TN1 10.4 K. Broadenings of the peaks in the M¨ossbauer spectrum wereobserved at temperatures below 6 K, which were due to the magnetic hyperfine fields transferredfrom the Yb magnetic moments. The evaluated transferred magnetic hyperfine field almost disappearsaround TN2. The anomalous temperature dependence of the transferred magnetic hyperfinefield reveals that the magnetic structure and the ordered magnetic moments of the Yb ions showcomplex temperature dependences at temperatures below TN1.