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Park, Hea Jung,So, Monica C.,Gosztola, David,Wiederrecht, Gary P.,Emery, Jonathan D.,Martinson, Alex B. F.,Er, Sü,leyman,Wilmer, Christopher E.,Vermeulen, Nicolaas A.,Aspuru-Guzik, Alá,n,S American Chemical Society 2016 ACS APPLIED MATERIALS & INTERFACES Vol.8 No.38
<P>We demonstrate that thin films of metal organic framework (MOF)-like materials, containing two perylenedlimides (PDICl4, PDIOPh2) and a squaraine dye (S1); can be fabricated by, layer-by-layer assembly (LbL). Interestingly, these LbL films absorb across the visible light region (400-750 nm) and facilitate directional energy transfer. Due to the high spectral overlap and oriented transition dipole moments of the donor (PDICl4 and PDIOPh2) and acceptor (S1) components, directional long-range energy transfer from the bluest to reddest absorber was successfully demonstrated in the multicomponent MOF-like films. These findings have significant implications for the development of solar energy conversion devices based on MOFs.</P>