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Jiang, Yi,Oh, Inseon,Joo, Se Hun,Buyukcakir, Onur,Chen, Xiong,Lee, Sun Hwa,Huang, Ming,Seong, Won Kyung,Kwak, Sang Kyu,Yoo, Jung-Woo,Ruoff, Rodney S. American Chemical Society 2019 JOURNAL OF THE AMERICAN CHEMICAL SOCIETY - Vol.141 No.42
<P>We report the synthesis and characterization of a two-dimensional (2D) conjugated Ni(II) tetraaza[14]annulene-linked metal organic framework (<B>NiTAA-MOF</B>) where <B>NiTAA</B> is a macrocyclic MN<SUB>4</SUB> (M = metal, N = nitrogen) compound. The structure of <B>NiTAA-MOF</B> was elucidated by Fourier-transform infrared, X-ray photoemission, and X-ray diffraction spectroscopies, in combination with density functional theory (DFT) calculations. When chemically oxidized by iodine, the insulating bulk <B>NiTAA-MOF</B> (σ < 10<SUP>-10</SUP> S/cm) exhibits an electrical conductivity of 0.01 S/cm at 300 K, demonstrating the vital role of ligand oxidation in the electrical conductivity of 2D MOFs. Magnetization measurements show that iodine-doped <B>NiTAA-MOF</B> is paramagnetic with weak antiferromagnetic coupling due to the presence of organic radicals of oxidized ligands and high-spin Ni(II) sites of the missing-linker defects. In addition to providing further insights into the origin of the induced electrical conductivity in 2D MOFs, both pristine and iodine-doped <B>NiTAA-MOF</B> synthesized in this work could find potential applications in areas such as catalase mimics, catalysis, energy storage, and dynamic nuclear polarization-nuclear magnetic resonance (DNP-NMR).</P> [FIG OMISSION]</BR>
Organic Radical-Linked Covalent Triazine Framework with Paramagnetic Behavior
Jiang, Yi,Oh, Inseon,Joo, Se Hun,Buyukcakir, Onur,Chen, Xiong,Lee, Sun Hwa,Huang, Ming,Seong, Won Kyung,Kim, Jin Hoon,Rohde, Jan-Uwe,Kwak, Sang Kyu,Yoo, Jung-Woo,Ruoff, Rodney S. American Chemical Society 2019 ACS NANO Vol.13 No.5
<P>The production of multifunctional pure organic materials that combine different sizes of pores and a large number of electron spins is highly desirable due to their potential applications as polarizers for dynamic nuclear polarization-nuclear magnetic resonance and as catalysts and magnetic separation media. Here, we report a polychlorotriphenylmethyl radical-linked covalent triazine framework (PTMR-CTF). Two different sizes of micropores were established by N<SUB>2</SUB> sorption and the presence of unpaired electrons (carbon radicals) by electron spin resonance and superconducting quantum interference device-vibrating sample magnetometer analyses. Magnetization measurements demonstrate that this material exhibits spin-half paramagnetism with a spin concentration of ∼2.63 × 10<SUP>23</SUP> spins/mol. We also determined the microscopic origin of the magnetic moments in PTMR-CTF by investigating its spin density and electronic structure using density functional theory calculations.</P> [FIG OMISSION]</BR>
Ying Yi,Shu-Bin Fang,Guan-Xia Xiong,Xian-Ren Wang,Hui-Ting Chen,Wan-Yi Huang,Li-Xuan Feng 대한이비인후과학회 2023 Clinical and Experimental Otorhinolaryngology Vol.16 No.1
Objectives. Reactive oxygen species in the stria vascularis (SV) of the cochlea may be involved in the pathogenesis of sen-sorineural hearing loss. However, the effects of oxidative stress on SV endothelial cells (SV-ECs) remain largely un-known, and no feasible in vitro cell culture model exists for the functional study of SV-ECs. Methods. We isolated primary SV-ECs from the SV of neonatal mice. The apoptosis-reducing effects of fibronectin in SV-ECs cultured with serum-free medium were determined using β-galactosidase staining and flow cytometry. SV-ECsincubated in serum-free medium were treated with various H2O2 concentrations to evaluate the effects of H2O2 ontheir viability. The secretome of SV-ECs treated with or without H2O2 (100 μM or 500 μM) was analyzed using high-resolution mass spectrometry. The function of the SV-EC secretome was evaluated by a macrophage assay. Results. We successfully isolated and characterized the SV-ECs. Treatment with H2O2 at concentrations up to 500 μM for2 hours and further incubation with serum-free medium in plates precoated with fibronectin showed no significanteffect on apoptosis. Compared to the control SV-ECs, the amount of differential proteins in the secretome of SV-ECsstimulated with 500 μM H2O2 was much higher than in those treated with 100 μM H2O2. Kyoto Encyclopedia ofGenes and Genomes and Gene Ontology analyses suggested that the proteins differentially expressed in SV-ECstreated with 500 μM H2O2 were involved in the regulation of multiple signaling pathways and cellular processes. Thesecretome of H2O2-stimulated SV-ECs exhibited significant pro-inflammatory effects on macrophages. Conclusion. We successfully established an in vitro serum-free culture method, identified the differential proteins releasedby oxidative stress-induced ECs and their functions, and revealed the pro-inflammatory effects of the secretome ofH2O2-stimulated SV-ECs. Therefore, SV-ECs might elicit immunoregulatory effects on bystander cells in the microen-vironment of oxidative stress-induced cochlea, especially cochlear macrophages.
Jiang, Yi,Ryu, Gyeong Hee,Joo, Se Hun,Chen, Xiong,Lee, Sun Hwa,Chen, Xianjue,Huang, Ming,Wu, Xiaozhong,Luo, Da,Huang, Yuan,Lee, Jeong Hyeon,Wang, Bin,Zhang, Xu,Kwak, Sang Kyu,Lee, Zonghoon,Ruoff, Rodn American Chemical Society 2017 ACS APPLIED MATERIALS & INTERFACES Vol.9 No.33
<P>Rational bottorritup construction of two-dimensional (2D) covalent or nonCovalent organic materials with precise structural control at the: atomic or molecular level remains a challenge. The design and synthesis of metal organic frameworks (MOFS) based on new building blocks is of great significance in achieving new types of 2D monolayer MOF films. Here, we demonstrate that a complexation between copper(II) ions and tri(beta-diketone) ligands yields a novel 2D MOF siyucture, either-inthe form of a powder.or.as a monolayer filth. It has been Characterized by Fourier transform infrared, Raman, ultraviolet-visible, X-ray photoelectron, and electron paramagnetic-resonance spectroscopies. Selected area electron diffraction and powder X-ray diffraction results show that the MOF is Crystalline and has a hexagonal structure. A MOF-based membrane has been prepared by vacuum filtration of an aqueous dispersion of the MOF powder onto a porous Anodisc filter having pore-size 0.02 mu m. The porous MOF membrane filters gold nanOparticies with a cutoff of similar to 2.4 nm.</P>
Hai-bo Huang,Yi-Jui Chiu,Xiao-xiong Jin 대한기계학회 2013 JOURNAL OF MECHANICAL SCIENCE AND TECHNOLOGY Vol.27 No.7
Tire wear negatively affects vehicle safety and riding comfort. Abnormal wear is more dangerous and wears tires out more quickly. In this paper, numerical and sensitivity analyses of polygonal wear caused by unstable vibration are presented. The model used for this study was based on the works of Sueoka. Tread self-excited vibration was analyzed in a quantitative sense, which was qualitatively different from the work of Sueoka. Wear was plotted on tire circumference visually. The mechanism governing polygonal tire wear was investigated as that both the polygonal wear and the standing wave are caused by two types of tread vibrations that only differ in the extent of the tread vibration. Sensitivity analysis shows that decreases in tread mass and stiffness and increases in tread damping lead to noticeable reductions in tire wear. This information could help tire manufacturers produce tires that exhibit less wear caused by tread vibration.
Freeze-Casting Produces a Graphene Oxide Aerogel with a Radial and Centrosymmetric Structure
Wang, Chunhui,Chen, Xiong,Wang, Bin,Huang, Ming,Wang, Bo,Jiang, Yi,Ruoff, Rodney S. American Chemical Society 2018 ACS NANO Vol.12 No.6
<P>We report the assembly of graphene oxide (G-O) building blocks into a vertical and radially aligned structure by a bidirectional freeze-casting approach. The crystallization of water to ice assembles the G-O sheets into a structure, a G-O aerogel whose local structure mimics turbine blades. The centimeter-scale radiating structure in this aerogel has many channels whose width increases with distance from the center. This was achieved by controlling the formation of the ice crystals in the aqueous G-O dispersion that grew radially in the shape of lamellae during freezing. Because the shape and size of ice crystals is influenced by the G-O sheets, different additives (ethanol, cellulose nanofibers, and chitosan) that can form hydrogen bonds with H<SUB>2</SUB>O were tested and found to affect the interaction between the G-O and formation of ice crystals, producing ice crystals with different shapes. A G-O/chitosan aerogel with a spiral pattern was also obtained. After chemical reduction of G-O, our aerogel exhibited elasticity and absorption capacity superior to that of graphene aerogels with “traditional” pore structures made by conventional freeze-casting. This methodology can be expanded to many other configurations and should widen the use of G-O (and reduced G-O and “graphenic”) aerogels.</P> [FIG OMISSION]</BR>
Establishing a Nomogram for Stage IA-IIB Cervical Cancer Patients after Complete Resection
Zhou, Hang,Li, Xiong,Zhang, Yuan,Jia, Yao,Hu, Ting,Yang, Ru,Huang, Ke-Cheng,Chen, Zhi-Lan,Wang, Shao-Shuai,Tang, Fang-Xu,Zhou, Jin,Chen, Yi-Le,Wu, Li,Han, Xiao-Bing,Lin, Zhong-Qiu,Lu, Xiao-Mei,Xing, H Asian Pacific Journal of Cancer Prevention 2015 Asian Pacific journal of cancer prevention Vol.16 No.9
Background: This study aimed to establish a nomogram by combining clinicopathologic factors with overall survival of stage IA-IIB cervical cancer patients after complete resection with pelvic lymphadenectomy. Materials and Methods: This nomogram was based on a retrospective study on 1,563 stage IA-IIB cervical cancer patients who underwent complete resection and lymphadenectomy from 2002 to 2008. The nomogram was constructed based on multivariate analysis using Cox proportional hazard regression. The accuracy and discriminative ability of the nomogram were measured by concordance index (C-index) and calibration curve. Results: Multivariate analysis identified lymph node metastasis (LNM), lymph-vascular space invasion (LVSI), stromal invasion, parametrial invasion, tumor diameter and histology as independent prognostic factors associated with cervical cancer survival. These factors were selected for construction of the nomogram. The C-index of the nomogram was 0.71 (95% CI, 0.65 to 0.77), and calibration of the nomogram showed good agreement between the 5-year predicted survival and the actual observation. Conclusions: We developed a nomogram predicting 5-year overall survival of surgically treated stage IA-IIB cervical cancer patients. More comprehensive information that is provided by this nomogram could provide further insight into personalized therapy selection.
A Health Management Service with Beacon-Based Identification for Preventive Elderly Care
Jian-Wei Li,Yi-Chun Chang,Min-Xiong Xu,De-Yao Huang 한국정보처리학회 2020 Journal of information processing systems Vol.16 No.3
Bluetooth low energy (BLE) beacon is an actively push-to-broadcast electronic signal and can be used for objectidentification. This paper uses such beacon-based identification and Internet of Things (IoT) technologies for theelder health management service system to simplify the user interfaces and steps for preventive elder care. Inthe proposed system, an elder’s family member, caregiver, or medical worker can conveniently and quicklyrecord daily health management information. Besides, through the statistics and analysis of the data on the backend of the system, it is helpful for the elderly to refer to the data of daily care management and futuremanagement trends. Similarly, it is also an essential reference data for system maintenance and the newpreventive health care services development.