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- 저자 : Xujie Yang (검색결과 4 건)
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Pressure-induced dramatic changes in organic–inorganic halide perovskites
Lü,, Xujie,Yang, Wenge,Jia, Quanxi,Xu, Hongwu Royal Society of Chemistry 2017 Chemical Science Vol.8 No.10
<▼1><P>We summarise cutting-edge discoveries and provide insights into the important theme of halide perovskites using pressure as a tuning tool.</P></▼1><▼2><P>Organic–inorganic halide perovskites have emerged as a promising family of functional materials for advanced photovoltaic and optoelectronic applications with high performances and low costs. Various chemical methods and processing approaches have been employed to modify the compositions, structures, morphologies, and electronic properties of hybrid perovskites. However, challenges still remain in terms of their stability, the use of environmentally unfriendly chemicals, and the lack of an insightful understanding into structure–property relationships. Alternatively, pressure, a fundamental thermodynamic parameter that can significantly alter the atomic and electronic structures of functional materials, has been widely utilized to further our understanding of structure–property relationships, and also to enable emergent or enhanced properties of given materials. In this perspective, we describe the recent progress of high-pressure research on hybrid perovskites, particularly regarding pressure-induced novel phenomena and pressure-enhanced properties. We discuss the effect of pressure on structures and properties, their relationships and the underlying mechanisms. Finally, we give an outlook on future research avenues in which high pressure and related alternative methods such as chemical tailoring and interfacial engineering may lead to novel hybrid perovskites uniquely suited for high-performance energy applications.</P></▼2>
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( Mulan Wei ),( Xujie Liu ),( Chunyu Cao ),( Jianlin Yang ),( Yafeng Lv ),( Jiaojiao Huang ),( Yanlin Wang ),( Ye Qin ) 생화학분자생물학회(구 한국생화학분자생물학회) 2018 BMB Reports Vol.51 No.11
Recent studies showed that the PD-1/PD-L1 checkpoint blockade is a dramatic therapy for melanoma by enhancing antitumor immune activity. Currently, major strategies for the PD-1/PD-L1 blockade have mainly focused on the use of antibodies and compounds. Seeking an alternative approach, others employ endogenous proteins as blocking agents. The extracellular domain of PD-1 (ePD1) includes the binding site with PD-L1. Accordingly, we constructed a PD-1-based recombinantly tailored fusion protein (dFv-ePD1) that consists of bivalent variable fragments (dFv) of an MMP-2/9-targeted antibody and ePD1. The melanoma-binding intensity and antitumor activity were also investigated. We found the intense and selective binding capability of the protein dFv-ePD1 to human melanoma specimens was confirmed by a tissue microarray. In addition, dFv-ePD1 significantly suppressed the migration and invasion of mouse melanoma B16-F1 cells, and displayed cytotoxicity to cancer cells in vitro. Notably, dFv-ePD1 significantly inhibited the growth of mouse melanoma B16-F1 tumor cells in mice and in vivo fluorescence imaging showed that dFv-ePD was gradually accumulated into the B16-F1 tumor. Also the B16-F1 tumor fluorescence intensity at the tumor site was stronger than that of dFv. This study indicates that the recombinant protein dFv-ePD1 has an intensive melanoma-binding capability and exerts potent therapeutic efficacy against melanoma. The novel format of the PD-L1-blocked agent may play an active role in antitumor immunotherapy. [BMB Reports 2018; 51(11): 572-577]
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Ag2O nanoparticle clusters coated with porous gelatin-g-PMMA copolymer
Ying Liu,Xiaoheng Liu,Xiaodong Wu,Xujie Yang,Lude Lu 한국물리학회 2010 Current Applied Physics Vol.10 No.3
Herein a special nanoparticle cluster coated with a porous copolymer is designed and prepared. At first,Ag2O nanoparticles (secondary particles) were fabricated in gelatin solution by a facile chemical approach. Then these nanoparticles were entrapped in a copolymerization system containing gelatin,methyl methacrylate (MMA), an initiator, and using water as a solvent. The nanoparticle clusters coated with porous gelatin-g-PMMA copolymer (Ag2O/gelatin-g-PMMA) were prepared by grafting methyl methacrylate onto gelatin, followed by coating solidification. One significant feature for our approach is that every Ag2O aggregated cluster has been coated with porous gelatin-g-PMMA copolymer film in a unique way, and the Ag2O nanoparticle could penetrate and escape from the coating freely in water by ultrasonication. As a result, this study provides a new approach to prepare monodispersed nanoparticles by ordered porous copolymers with controlled releasing.
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Lu Wang,Xiaoheng Liu,Xin Wang,Xujie Yang,Lude Lu 한국물리학회 2010 Current Applied Physics Vol.10 No.6
Mesoporous Co3O4 microspheres with unique crater-like morphology were obtained by utilizing the mesoporous silica material MCM-41 as a template. The analysis results of N2 adsorptionedesorption measurement indicate that the product has a large BrunauereEmmetteTeller (BET) surface area of 60 m2 g-1 and a narrow pore size distribution centering around 3.7 nm. Its electrochemical properties were investigated by cyclic voltammetry (CV) and electrochemical impedance spectroscopy (EIS)measurements. The findings reveal that this novel morphology material has a smaller inner resistance of about 0.4 U and a higher onset frequency of 550 Hz. This material can provide a high specific capacitance of 102 F g-1 and a large capacity retention of 74% in 500 continuous cycles test at a sweep rate of 3 mV s-1. More significantly, the mass loading of electroactive species can reach as large as 2 mg cm-2, which is one order of magnitude larger than common amount used.
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