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- 저자 : Tangfu Xiao (검색결과 2 건)
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Nana Wang,Xingjian Xu,Li Yang,Lizhu Yuan,Tangfu Xiao,Haiyan Li,Hongwen Yu 한국공업화학회 2018 Journal of Industrial and Engineering Chemistry Vol.66 No.-
A sponge-type composite adsorbent xanthate-modified chitosan @ titanate nanotubes (XCTS@TNTs) was prepared via a simple and low-cost procedure, and its adsorption capacity was evaluated in batch and continuous plate column systems. The three-dimensional network macroporous structure made it easy to separate from the solution and suitable for the column-based treatment. The excellent adsorption capacity of Pb(II) was as high as 342.47 mg/g and could be obtained in wide ranges of pH and temperature. Interestingly, XCTS@TNTs exhibited outstanding selectivity for Pb(II) rather than other divalent heavy metal ions. Adsorption mechanism was elucidated by the FTIR and XPS analyses. The column adsorption results indicated that the treatment effect was proportional to bed height and inversely to flow rate and influent concentration. XCTS@TNTs was remarkably effective in the removal of Pb(II) from actual industrial effluents to meet the discharge requirements and contributed to the recovery of Pb(II). The treatment volumes of simulated actual battery wastewater and smelting effluent by 2.40 g XCTS@TNTs were as high as 6360 and 49584 mL for Pb(II) with the concentration of 30.55 and 4.49 mg/L, respectively. This work developed a highly practical process for removing heavy metal ions from practical wastewaters.
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Mingxia Yu,Huosheng Li,Keke Li,Yuting Li,Fengli Liu,Gaosheng Zhang,Tangfu Xiao,Ping Zhang,Hongguo Zhang,Jianyou Long 한국섬유공학회 2022 Fibers and polymers Vol.23 No.2
Decolorization and organic degradation of wastewater containing multiple dyes are still challenging inwastewater treatment. Magnetic biochar coupled with advanced oxidation is a potential solution to this issue. In this study,a series of magnetite-based biochar composites (Fe3O4@C) was prepared and compared for the removal of mixed dyes,including methyl orange (MO), rhodamine B (RhB), methylene blue (MB), and an organic macromolecule, humic acid(HA). The pyrolysis of watermelon rinds followed by precipitation of Fe3O4 onto the biochar was selected as the optimummethod to prepare an adsorbent and catalyst to couple binary oxidants (hypochlorite and persulfate) for color and totalorganic carbon removal. Persulfate was prone to degrade HA and MB, while hypochlorite was inclined to oxidize MO andRhB. Fe3O4@C exhibited better dye removal performance in coupling with binary oxidants than with a single oxidant. Formixed dye solutions with an initial concentration of 50 mg/l for each dye, the highest TOC (57.24±3.17 %) and the colorremoval efficiencies (94.13±1.68 %) for the mixed dye solution were achieved at a sorbent dosage of 1 g/l and an oxidantdosage of 5 mmol/l for both hypochlorite and persulfate. Multiple free radicals, including hydroxyl radicals, sulfateradicals, and hypochlorite-induced radicals, play critical roles in the degradation of mixed dyes and color removal. Theregeneratibility and reutilization of the magnetic Fe3O4@C composite were effective and stable. The results obtained inthis study show that the combined Fe3O4@C and binary oxidants technique is promising for the treatment of multi-dyewastewater.
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