http://chineseinput.net/에서 pinyin(병음)방식으로 중국어를 변환할 수 있습니다.
변환된 중국어를 복사하여 사용하시면 됩니다.
SURFACE WAVES IN SOLAR GRANULATION OBSERVED WITH SUNRISE
Roth, M.,Franz, M.,Bello Gonzá,lez, N.,Martí,nez Pillet, V.,Bonet, J. A.,Gandorfer, A.,Barthol, P.,Solanki, S. K.,Berkefeld, T.,Schmidt, W.,del Toro Iniesta, J. C.,Domingo, V.,Knö,lker IOP Publishing 2010 ASTROPHYSICAL JOURNAL LETTERS - Vol.723 No.2
New insights in the formation processes of Pu(IV) colloids
Walther, Clemens,Rothe, Jö,rg,Brendebach, Boris,Fuss, Markus,Altmaier, Marcus,Marquardt, Christian M.,Bü,chner, Sebastian,Cho, Hye-Ryun,Yun, J.-I.,Seibert, Alice De Gruyter Oldenbourg 2009 RADIOCHIMICA ACTA Vol.97 No.4
<P><B>Abstract</B></P><P>The high tendency of tetravalent plutonium to form polymeric complexes and colloids is well known but the exact processes underlying their formation are still controversially discussed. In the present work, the nucleation of small polynuclear hydroxide complexes,<I>i.e.</I>, ionic species containing more than one Pu ion, their aggregation and formation of larger colloids (polymers exceeding some 5 nm in size) and finally ripening processes of freshly formed amorphous Pu(IV) colloids towards more crystalline particles are investigated by use of a combination of various spectroscopic techniques. By electrospray mass-spectrometry small polymers such as dimers, trimers and tetramers containing mixed oxidation states of Pu were observed. These polymers might be responsible for the equilibration between the Pu(III)/Pu(IV) and the plutonyl species Pu(V)/Pu(VI) even in dilute solutions in the absence of colloids or precipitates.</P>
Fine structure of the isoscalar giant quadrupole resonance inSi28andAl27
Usman, I. T.,Buthelezi, Z.,Carter, J.,Cooper, G. R. J.,Fearick, R. W.,Fö,rtsch, S. V.,Fujita, H.,Fujita, Y.,von Neumann-Cosel, P.,Neveling, R.,Papakonstantinou, P.,Pysmenetska, I.,Richter, A.,Roth American Physical Society 2016 Physical Review C Vol.94 No.2
<P>The isoscalar giant quadrupole resonance in Si-28 and Al-27 has been investigated with high-energy-resolution proton inelastic scattering at E-p = 200 MeV and at scattering angles close to the maximum of Delta L = 2 angular distributions with the K600 magnetic spectrometer of iThemba LABS, South Africa. Characteristic scales are extracted from the observed fine structure with a wavelet analysis and compared for Si-28 with random-phase approximation and second random phase approximation calculations with an interaction derived from the Argonne V18 potential by a unitary transformation. A recent extension of the method to deformed nuclei provides the best description of the data, suggesting the significance of Landau damping.</P>
Lee, Jun-Yeop,Vespa, Marika,Gaona, Xavier,Dardenne, Kathy,Rothe, Jö,rg,Rabung, Thomas,Altmaier, Marcus,Yun, Jong-Il De Gruyter 2017 RADIOCHIMICA ACTA Vol.105 No.3
<P><B>Abstract</B></P><P>The formation of ternary Mg-UO<SUB>2</SUB>-CO<SUB>3</SUB>complexes under weakly alkaline pH conditions was investigated by time-resolved laser fluorescence spectroscopy (TRLFS) and extended X-ray absorption fine structure (EXAFS) and compared to Ca-UO<SUB>2</SUB>-CO<SUB>3</SUB>complexes. The presence of two different Mg-UO<SUB>2</SUB>-CO<SUB>3</SUB>complexes was identified by means of two distinct fluorescence lifetimes of 17±2 ns and 51±2 ns derived from the multi-exponential decay of the fluorescence signal. Slope analysis in terms of fluorescence intensity coupled with fluorescence intensity factor as a function of log [Mg(II)] was conducted for the identification of the Mg-UO<SUB>2</SUB>-CO<SUB>3</SUB>complexes forming. For the first time, the formation of both MgUO<SUB>2</SUB>(CO<SUB>3</SUB>)<SUB>3</SUB><SUP>2−</SUP>and Mg<SUB>2</SUB>UO<SUB>2</SUB>(CO<SUB>3</SUB>)<SUB>3</SUB>(aq) species was confirmed and the corresponding equilibrium constants were determined as log β<SUP>0</SUP><SUB>113</SUB>=25.8±0.3 and log β<SUP>0</SUP><SUB>213</SUB>=27.1±0.6, respectively. Complementarily, fundamental structural information for both Ca-UO<SUB>2</SUB>-CO<SUB>3</SUB>and Mg-UO<SUB>2</SUB>-CO<SUB>3</SUB>complexes was gained by extended EXAFS revealing very similar structures between these two species, except for the clearly shorter U-Mg distance (3.83 Å) compared with U-Ca distance (4.15 Å). These results confirmed the inner-sphere character of the Ca/Mg-UO<SUB>2</SUB>-CO<SUB>3</SUB>complexes. The formation constants determined for MgUO<SUB>2</SUB>(CO<SUB>3</SUB>)<SUB>3</SUB><SUP>2−</SUP>and Mg<SUB>2</SUB>UO<SUB>2</SUB>(CO<SUB>3</SUB>)<SUB>3</SUB>(aq) species indicate that ternary Mg-UO<SUB>2</SUB>-CO<SUB>3</SUB>complexes contribute to the relevant uranium species in carbonate saturated solutions under neutral to weakly alkaline pH conditions in the presence of Mg(II) ions, which will induce notable influences on the U(VI) chemical species under seawater conditions.</P>