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Yee Hwa Sehlleier,Sascha Dobrowolny,Lisong Xiao,Angelika Heinzel,Christof Schulz,Hartmut Wiggers 한국공업화학회 2017 Journal of Industrial and Engineering Chemistry Vol.52 No.-
The processing towards Si/C composites, components and synthesis parameters were selected based onthe concept of Hansen solubility parameters (HSP). Si/polymer composites were generated throughmodified bulk polymerization and subsequent pyrolysis transformed the polymer into the desired porouscarbon matrix. Coulombic efficiencies (CE) in excess of 76% after thefirst cycle and 99.95% after solidelectrolyte interphase (SEI) formation have been achieved. A notably high specific delithiation capacity ofaround 1600 mAh/g with an extremely stable cycling performance even after 400 cycles is obtained. Thisscalable and economical synthesis approach is readily applicable to the commercial production of anodematerials.