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Selective surface functionalization at regions of high local curvature in graphene
Wu, Qingzhi,Wu, Yaping,Hao, Yufeng,Geng, Jianxin,Charlton, Matthew,Chen, Shanshan,Ren, Yujie,Ji, Hengxing,Li, Huifeng,Boukhvalov, Danil W.,Piner, Richard D.,Bielawski, Christopher W.,Ruoff, Rodney S. The Royal Society of Chemistry 2013 Chemical communications Vol.49 No.7
<P>Monolayer graphene was deposited on a Si wafer substrate decorated with SiO<SUB>2</SUB> nanoparticles (NPs) and then exposed to aryl radicals that were generated <I>in situ</I> from their diazonium precursors. Using micro-Raman mapping, the aryl radicals were found to selectively react with the regions of graphene that covered the NPs. The enhanced chemical reactivity was attributed to the increased strain energy induced by the local mechanical deformation of the graphene.</P> <P>Graphic Abstract</P><P>Due to the increased strain energy caused by local mechanical deformation, aryl radicals were found to selectively react with regions of graphene that were curved by underlying SiO<SUB>2</SUB> nanoparticles. <IMG SRC='http://pubs.rsc.org/services/images/RSCpubs.ePlatform.Service.FreeContent.ImageService.svc/ImageService/image/GA?id=c2cc36747e'> </P>
AN IMPROVED METHOD FOR TRANSFERRING GRAPHENE GROWN BY CHEMICAL VAPOR DEPOSITION
YUJIE REN,CHAOFU ZHU,WEIWEI CAI,HUIFENG LI,YUFENG HAO,YAPING WU,SHANSHAN CHEN,QINGZHI WU,RICHARD D. PINER,RODNEY S. RUOFF 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2012 NANO Vol.7 No.1
In this paper, we report an improved transfer of graphene by directly picking up the graphene with target substrates and the comparison of such transferred graphene samples with other graphene samples transferred by the commonly used "PMMA-based transfer" method. Raman spectroscopy studies show that this "direct transfer method" does not degrade the graphene structure and field effect transistor measurements show that it does not introduce any extra doping in graphene; in contrast, PMMA-based transfer samples have strong n-type doping. We also find that graphene samples achieved by this direct transfer method show higher mobility than graphene obtained from the PMMA-based transfer method.