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A Computational Meta-Analysis of UCl<sub>3</sub> Cyclic Voltammograms in LiCl-KCl Electrolyte
Cumberland, Riley M.,Yim, Man-Sung The Electrochemical Society 2014 Journal of the Electrochemical Society Vol.161 No.4
<P>As a way to characterize the values of key parameters for modeling electrochemical transport of elements in a molten salt system, a meta-analysis of CV reduction peaks for UCl<SUB>3</SUB> in LiCl-KCl eutectic was performed. Published CV data was fit using least squares fitting software coupled with electrochemical simulation software. The analysis yielded estimates of apparent standard potential, the diffusion coefficient, and the exchange current density for each reaction. The results for the UCl<SUB>3</SUB> reduction peak matched well with existing data.</P>
ANALYSIS OF EQUILIBRIUM METHODS FOR THE COMPUTATIONAL MODEL OF THE MARK-IV ELECTR OREFINER
RILEY CUMBERLAND,ROBERT HOOVER,SUPATHORN PHONGIKAROON,임만성 한국원자력학회 2011 Nuclear Engineering and Technology Vol.43 No.6
Two computational methods for determining equilibrium states for the Mark-IV electrorefiner (ER) have been assessed to improve the current computational electrorefiner model developed at University of Idaho. Both methods were validated against measured data to better understand their effects on the calculation of the equilibrium compositions in the ER. In addition, a sensitivity study was performed on the effect of specific unknown activity coefficients—including sodium in molten cadmium, zirconium in molten cadmium, and sodium chloride in molten LiCl-KCl. Both computational methods produced identical results, which stayed within the 95% confidence interval of the experimental data. Furthermore, sensitivity to unavailable activity coefficients was found to be low (a change in concentration of less than 3 ppm).
ANALYSIS OF EQUILIBRIUM METHODS FOR THE COMPUTATIONAL MODEL OF THE MARK-IV ELECTR OREFINER
Cumberland, Riley,Hoover, Robert,Phongikaroon, Supathorn,Yim, Man-Sung Korean Nuclear Society 2011 Nuclear Engineering and Technology Vol.43 No.6
Two computational methods for determining equilibrium states for the Mark-IV electrorefiner (ER) have been assessed to improve the current computational electrorefiner model developed at University of Idaho. Both methods were validated against measured data to better understand their effects on the calculation of the equilibrium compositions in the ER. In addition, a sensitivity study was performed on the effect of specific unknown activity coefficients-including sodium in molten cadmium, zirconium in molten cadmium, and sodium chloride in molten LiCl-KCl. Both computational methods produced identical results, which stayed within the 95% confidence interval of the experimental data. Furthermore, sensitivity to unavailable activity coefficients was found to be low (a change in concentration of less than 3 ppm).