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Resonance Raman intensity analysis of an intramolecular charge-transfer process
Sarah L. Howell,Keith C. Gordon,Mark R. Waterland 한국물리학회 2006 Current Applied Physics Vol.6 No.3
We present an analysis of the resonance Raman intensities of an intramolecular charge-transfer transition using a time-domain for-mulation of the Raman scattering process. This analysis provides mode-specic reorganization energies for the vibrational modes thatcouple to the photoinduced charge-transfer event. In addition, the absolute magnitude of the resonance Raman intensities allows thesurrounding solvent contribution to the reorganization energy to also be determined. The analysis demonstrates that for the intramo-tion energies.