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Liu Guijing,Shi Yanying,Wang Lei,Song Yadong,Gao Shanmin,Liu Dong,Fan Leqing 한국탄소학회 2020 Carbon Letters Vol.30 No.4
Polypyrrole (PPy) decorated on reduced graphene oxide (rGO) flms is successfully prepared with pyrrole (Py) monomers and rGO through one-step combining oxidation with polymerization reaction. Compared with the pure individual compo�nents, rGO/PPy compound turns out better electrochemical characteristics owing to the introduction of rGO sheets, which improves the specifc surface area and the conductivity of composite material. When the amount of rGO is 10% of the total, the rGO/PPy compound delivers the best capacitance of 389.3 F g−1 at 1.0 A g−1 in a three-electrode system and 266.8 F g−1 at 0.25 A g−1 in the symmetric supercapacitor system. In addition, asymmetric device (rGO/PPy//AC) has been success�fully fabricated using optimized rGO/PPy compound as positive electrode, activated carbon as negative electrode (AC) and 1 M Na2SO4 aqueous solution as electrolyte. The device obtains long cycle stability under the high-voltage region from 0 to 1.6 V, meanwhile displaying the satisfed energy density of 19.7 Wh kg−1 at 478.1 W kg−1. Besides, the rGO/PPy//AC device presents satisfactory rate capability and long life time.