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        Effect of Partial Magnetic Order on Resistivity and Thermopower of Ho(Co1−xAlx)2 Alloys

        T. Nakama,C. Zukeran,A. Nakamura,A. Teruya,S. Hirakawa,S. Watanabe,Y. Hiranaka,M. Takeda,M. Hedo,K. Yagasaki,Y. Takaesu,K. Uchima,A. T. Burkov 한국물리학회 2013 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.63 No.3

        The electrical resistivity and the thermopower S of Ho(Co1−xAlx)2 alloys (x = 0 to 0.2) weremeasured at temperatures from 2 K to 300 K in magnetic fields up to 10 T. While (T) and S(T)of pure HoCo2 reveal abrupt changes at the magnetic ordering temperature TC, indicating a firstordertransition, the temperature variations of both properties across the ordering temperature inHo(Co1−xAlx)2 alloys clearly show that the type of magnetic transition changes under substitutionof Al for Co from first order to second order around x 0.06. (T) of the Al-substituted samples (x= 0.15 and 0.2) has a very unusual variation at temperatures below TC: in contrast to the expectedand usually-observed decrease of (T), the resistivity of Ho(Co1−xAlx)2 alloys (x = 0.15 and 0.2)increases at temperatures below TC. Moreover, the magnetoresistance of these alloys is positivearound TC; this is also in a sharp contrast to the usually observed negative magnetoresistance. We show that the anomalous resistivity and magnetoresistance in these alloys are related to themetamagnetic instability of the Co 3d subsystem and to the fluctuating local magnetic susceptibilitydue to atomic substitution. Due to this fluctuating local magnetic susceptibility, the uniformexchange field of 4f moments induces a non-uniform polarization of the 3d system, with staticspatial fluctuations of the local magnetization. This static magnetic disorder gives an additionalcontribution (m) to the electrical resistance in the alloys at temperatures below TC. The degreeof this disorder changes with decreasing temperature, resulting in specific variation of m withtemperature.

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