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X-ray Absorption and Photoemission Spectroscopy Study of Nd½A½Mn₁-yCryO₃ (A=Ca, Sr)
J.-S. Kang,J. H. Kim,S. W. Han,K. H. Kim,E. J. Choi,A. Sekiyama,S. Kasai,S. Suga,T. Kimura 한국자기학회 2003 Journal of Magnetics Vol.8 No.4
Valence states and electronic structures of Cr-doped Nd½A½MnO₃ (NAMO; A=Ca, Sr) manganites have been investigated using x-ray absorption spectroscopy (XAS) and high-resolution photoemission spectroscopy (PES). All the Cr-doped NAMO systems exhibit the clear metallic Fermi edges in the Mn e_g PES spectra near E_F. The spectral intensity at E_F is higher for Cr-doped Nd½Sr½MnO₃ (NSMO) than for Cr-doped Nd½Ca½MnO₃ (NCMO), reflecting the stronger metallic nature for NSMO than for NCMO. The measured Cr 2p XAS spectra are found to be very similar to that of Cr₂O₃, indicating that Cr ions in Cr-doped NAMO are in the trivalent Cr³+ states (t³_(2g)). The Cr 2p XAS data are consistent with the Cr 3d PES spectra located at ~1.3 eV below EF and having no emission near E_F.
H. Fujiwara,Y. Nakatani,H. Aratani,Y. Kanai-Nakata,K. Yamagami,S. Hamamoto,T. Kiss,A. Sekiyama,A. Tanaka,T. Ebihara,Y. Saitoh 한국물리학회 2023 새물리 Vol.73 No.12
We have performed the soft x-ray absorption spectroscopy (XAS) on the heavy fermion superconductor CeNi₂Ge₂ to examine the local 4f electronic structures. The XAS spectra are qualitatively explained by the ionic calculation, indicating the localized character of the 4f states, while the sizable cf-hybridization effects are also observed in the XAS spectra and those magnetic circular dichroism. In addition, the temperature dependence of linear dichroism (LD) in the XAS spectra indicates that the ground state symmetry is Γ<SUB>7</SUB>, and the excited states with Γ<SUB>6</SUB> symmetry is above 390 K.