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Unconventional anomalous Hall effect from antiferromagnetic domain walls of Nd2Ir2O7 thin films
Kim, Woo Jin,Gruenewald, John H.,Oh, Taekoo,Cheon, Sangmo,Kim, Bongju,Korneta, Oleksandr B.,Cho, Hwanbeom,Lee, Daesu,Kim, Yoonkoo,Kim, Miyoung,Park, Je-Geun,Yang, Bohm-Jung,Seo, Ambrose,Noh, Tae Won American Physical Society 2018 Physical Review B Vol.98 No.12
Souri, M.,Kim, B. H.,Gruenewald, J. H.,Connell, J. G.,Thompson, J.,Nichols, J.,Terzic, J.,Min, B. I.,Cao, G.,Brill, J. W.,Seo, A. American Physical Society 2017 Physical review. B Vol.95 No.23
<P>We have investigated the electronic and optical properties of (Sr1-xCax)(2)IrO4 (x = 0-0.375) and (Sr1-yBay)(2)IrO4 (y = 0-0.375) epitaxial thin films, in which the bandwidth is systematically tuned via chemical substitutions of Sr ions by Ca and Ba. Transport measurements indicate that the thin-film series exhibits insulating behavior, similar to the J(eff) = 1/2 spin-orbit Mott insulator Sr2IrO4. As the average A-site ionic radius increases from (Sr1-xCax)(2)IrO4 to (Sr1-yBay)(2)IrO4, optical conductivity spectra in the near-infrared region shift to lower energies, which cannot be explained by the simple picture of well-separated J(eff) = 1/2 and J(eff) = 3/2 bands. We suggest that the two-peak-like optical conductivity spectra of the layered iridates originates from the overlap between the optically forbidden spin-orbit exciton and the intersite optical transitions within the J(eff) = 1/2 band. Our experimental results are consistent with this interpretation as implemented by a multiorbital Hubbard model calculation: namely, incorporating a strong Fano-like coupling between the spin-orbit exciton and intersite d-d transitions within the J(eff) = 1/2 band.</P>