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      저자 : Chentao Zou (검색결과 2 건)
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        Preparation of Bi/Bi2MoO6 Plasmonic Photocatalyst with High Photocatalytic Activity Under Visible Light Irradiation

        Chentao Zou,Zhiyuan Yang,Mengjun Liang,Yunpeng He,Yun Yang,Shuijin Yang 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2018 NANO Vol.13 No.11

        Bi metal deposited on Bi2MoO6 composite photocatalysts have been successfully synthesized via a simple reduction method at room temperature with using NaBH4 as the reducing agent. The photocatalytic activity of the composite was evaluated by degradation of rhodamine B (RhB) and bisphenol A (BPA) solution under visible light. The rate constant of Bi/Bi2MoO6 composite to RhB is 10.8 times that of Bi2MoO6, and the degradation rate constant of BPA is 6.9 times of that of Bi2MoO6. Nitrogen absorption–desorption isotherm proved that the increase of specific surface area is one of the reasons for the improvement of photocatalytic degradation activity of Bi/Bi2MoO6 composites. The higher charge transfer efficiency of Bi/Bi2MoO6 is found through the characterization of the photocurrent and impedance, which are attributed to the surface plasmon resonance (SPR) effect produced by the introduction of the metal Bi monomer in the composite. Free radical capture experiments proved that cavitation is the main active species. Based on the above conclusions, a possible mechanism of photocatalytic degradation is proposed.

      • KCI등재

        In Situ Fabrication of TiO2/Bi3.64Mo0.36O6.55 Nanocomposite with High Visible-Light-Driven Photocatalytic Efficiency

        Zhiyuan Yang,Junjie Wang,Lu Chen,Mengjun Liang,Yulin Xu,Chentao Zou,Xiaoxia Liu,Shuijin Yang 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2017 NANO Vol.12 No.5

        In this work, we developed a simple hydrothermal method toward the fabrication of TiO2/ Bi3.64Mo0.36O6.55 heterostructure, which had superior photocatalytic performance for degrading of RhB under visible light irradiation. The as-prepared samples were characterized by X-ray diffraction (XRD), field emission scanning electron microscope (FESEM), high-resolution transmission electron microscopy (HRTEM), UV-Vis diffuse reflectance spectroscopy (DRS) and photoelectrochemical measurements. The optimal composite with 15 wt.% TiO2/Bi3.64Mo0.36O6.55 (TBMO3) exhibits a much higher photocatalytic activity than that of Bi3.64Mo0.36O6.55 and P25 by degradation of RhB under visible light irradiation within 20 min. The enhanced performance of TBMO3 is predominantly attributed to the synergistic effect both in the higher surface area and the improved separation of photogenerated charge carriers between the two semiconductors. Recycling experiments indicated that TiO2/Bi3.64Mo0.36O6.55 photocatalysts had excellent cycle performance and stability. The photocatalytic mechanism of nanocomposite photocatalysts was proposed, which is confirmed by the active species trapping experiments and photoluminescence tests.

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