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DFT and TD-DFT study on structure and properties of organic dye sensitizer TA-St-CA
Cai-Rong Zhang,Zi-Jiang Liu,Yu-Hong Chen,Hong-Shan Chen,You-Zhi Wu,WangJun Feng,Dao-Bin Wang 한국물리학회 2010 Current Applied Physics Vol.10 No.1
The geometry, electronic structure, polarizability and hyperpolarizability of organic dye sensitizer TA-St-CA, which contains a π-conjugated oligo-phenylenevinylene unit with an electron donor.acceptor moiety, was studied using density functional theory (DFT), and the electronic absorption spectrum was investigated via time-dependent DFT (TD-DFT) with several hybrid functionals. The calculated geometry indicates that the strong conjugated effects are formed in the dye. The TD-DFT results show that the hybrid functional PBE1PBE and MPW1PW91 are more suitable than B3LYP for calculating electronic absorption spectra. The features of electronic absorption spectra were assigned on account of the qualitative agreement between the experiment and the calculations. The absorption bands in visible and near-UV region are related to photoinduced electron transfer processes, and the diphenylaniline group is major chromophore that contributed to the sensitization, and the interfacial electron transfer are electron injection processes from the excited dyes to the semiconductor conduction band. Compared with the similar dye D5, the good performance of TA-St-CA in dye-sensitized solar cells may be resulted from the higher energy level of the lowest unoccupied molecular orbital and the larger oscillator strengths for the most excited states with intramolecular electron transfer character.
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Research of the Exciting Current Detection Method of MCR
Wang Jun,Wei Liangliang,Chen Feng,Nie Dexin,Lu Wenhua 보안공학연구지원센터 2016 International Journal of Multimedia and Ubiquitous Vol.11 No.5
Magnetic valve controllable reactor (MCR) is a kind of dynamic reactive power compensation device. The exciting current of MCR is one of the important indexes of operating condition of MCR. This paper firstly analyzed the principle of MCR, and deduced the relationship between the exciting current and the output current, verified by MATLAB/SIMULINK. And then an effective method to detect the exciting current was proposed by this paper. The method has the advantages of optical fiber isolation, high detection precision, strong anti-interference, etc. Finally, a 220v/1200var MCR was experimented in detail. The results demonstrate the accuracy of the theoretical analysis.
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