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Xiaogang Zheng,Fuyan Kang,Congying Huang,Sihao Lv,JinYang Zhang,Hao Peng 한국공업화학회 2020 Journal of Industrial and Engineering Chemistry Vol.88 No.-
ZnS–ZnO–Sm2O3 (Zn–Sm–XY) composites were prepared via the high-temperature calcination of coreshellstructured ZnS@Sm2O3 for the enhanced photocatalytic degradation of dyes and antibiotics invisible light region. Effects of calcined temperature, Sm2O3 content, pH value, contaminantconcentration, and inorganic ions on the photocatalytic activity were investigated. Ternary Zn–Smcomposites exhibit the excellent photocatalytic activity for the visible light driven degradation oftetracycline hydrochloride. Among these composites, Zn–Sm–2B prepared via the heat-treatment ofZnS–Sm2O3 at 673 K shows the best photocatalytic activity for the removal of tetracycline hydrochloride. The enhanced photocatalytic activity of Zn–Sm–2B is also achieved for the visible light drivendegradation of methyl orange, methylene blue, and rhodamine B within 20 min. In addition, Zn–Sm–6Ccalcined from Zn–Sm–C at 1073 K as well as Zn–Sm–2B exhibits excellent photocatalytic activity. OH andO2radicals are vital for the enhanced photocatalytic activity of Zn–Sm–2B and Zn–Sm–2B in visiblelight region, respectively. The lattice defects, sulfur vacancies, and oxygen vacancies facilitate the efficientcharge transfer and the rapid separation of electron-hole pairs at the junction interface of Zn–Sm–2B.