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Congcong Li,Ruiqi Li,Yuhang Wang,Runhan Niu,Qilong Guo,Changsen Zhang 한국공업화학회 2023 Journal of Industrial and Engineering Chemistry Vol.126 No.-
A series of manganese-based oxide catalysts were synthesized by the hydrothermal method. By adjustingthe doping amounts of W and Cu in the system to study the catalytic performance of transition metaldopedmanganese oxides on soot combustion. They were deeply studied through various characterizationsand theoretical calculations. The results show that Wand Cu doping modifications can significantlyimprove the activity of manganese-based oxides in soot oxidation. W-Cu0.1/MnOx prepared by comodificationofWand Cu at 395 C can convert 90% of soot into CO2. The multiple characterization resultsshow that by adjusting the doping amount of copper and tungsten, the nano-flower-like morphology canbe obtained and the crystal plane can be reconstructed, which is helpful to increase the specific surfacearea, Mn3+ content, and oxygen vacancy content. The theoretical calculation results show that the oxygenvacancy on the surface of the catalyst shows the ability to activate O2 and H2O, and they show noncompetitiveadsorption. In addition, W-Cu0.1/MnOx has a good application prospect in the catalytic oxidationof soot because of its excellent catalytic stability. This work provides a reference for the designand preparation of non-noble metal-based catalysts for the elimination of soot particles from dieselengine exhaust.
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