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- 저자 : L.S. Taura (검색결과 1 건)
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Abdullahi Lawal,A. Shaari,R. Ahmed,L.S. Taura 한국물리학회 2018 Current Applied Physics Vol.18 No.5
The rapid demand of photodetector is increasing day by day due to its versatility of applications that affect our lives. However, it is still very challenging to produce low-cost high-performance broadband photo-detector that can detect light from near infrared to the ultraviolet frequency range for medical diagnosis and visible light communication applications. Regarding this, low-cost antimony selenide (Sb2Se3), with direct energy gap and strong light absorption over a wider range from near infrared to ultraviolet frequency, is considered a promising candidate material for such kind of applications. Therefore, to expose its hidden potential, detailed analysis of its structural, electronic and optical properties is very essential. To accomplish this purpose, different schemes of the first-principles calculations are used in this study. Structural properties of Sb2Se3 are calculated by first-principles methods realized within density functional theory (DFT) framework. Whereas, to compute the quasiparticle (QP) band structure, excitonic and optical properties, many-body perturbation theory (MBPT) based on oneshot GW (G0W0) and Bethe-Salpeter equation (G0W0-BSE) approaches are used. Our DFT calculations show that Wu-Cohen GGA (WC-GGA) reproduces lattice parameters of Sb2Se3 material consistent with the experimental measurements. Similarly, G0W0 calculations confirm the Sb2Se3 a direct bandgap energy material of 1.32 eV and show good agreement with the experimental results. Similarly, the results on the optical properties of Sb2Se3 with the inclusion of electron-hole interaction show that the exciton energy of the material is 1.28eV while its corresponding plasma energy is 10.86 eV. These values show that the investigated material can absorb photons from near infrared to ultraviolet wavelengths. It is, therefore, anticipated that this material will be useful for new-generation optoelectronic applications from near infrared to ultraviolet wavelengths.
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