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        Spin-Injection Dynamics and Eects of Spin Relaxation in Self-Assembled Quantum Dots of CdSe

        T. Furuta,K. Hyomi,I. Souma,Y. Oka,A. Murayama,D. Dagnelund,I. A. Buyanova,W. M. Chen 한국물리학회 2008 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.53 No.1

        We study the spin injection dynamics and the eects of spin relaxation in self-assembled quantum dots (QDs) of CdSe coupled with a diluted magnetic semiconductor (DMS) layer of ZnMnSe, where spin-polarized excitons can be injected from the DMS into the QDs because of the potential dierence. The degree of circular polarization, P, of excitonic photoluminescence (PL) at 5 T in the coupled QDs shows a rapid increase with increasing delay time after a linearly polarized pulse excitation, indicating the spin-injection dynamics. The P value tends to decay gradually because of the exciton-spin relaxation in the QDs after the spin injection. The spin-polarized excitons in the QD ensemble migrate simultaneously from QDs with higher exciton energies to those with lower exciton energies. This inter-dot transfer of excitons also aects the P value in the lower energy region of the QD-emission band because the excitons lose their spin polarizations due to the spin relaxation in the dots during the migration. The detailed analysis for the exciton-spin transfer is presented in a coupled QD system after spin injection. We study the spin injection dynamics and the eects of spin relaxation in self-assembled quantum dots (QDs) of CdSe coupled with a diluted magnetic semiconductor (DMS) layer of ZnMnSe, where spin-polarized excitons can be injected from the DMS into the QDs because of the potential dierence. The degree of circular polarization, P, of excitonic photoluminescence (PL) at 5 T in the coupled QDs shows a rapid increase with increasing delay time after a linearly polarized pulse excitation, indicating the spin-injection dynamics. The P value tends to decay gradually because of the exciton-spin relaxation in the QDs after the spin injection. The spin-polarized excitons in the QD ensemble migrate simultaneously from QDs with higher exciton energies to those with lower exciton energies. This inter-dot transfer of excitons also aects the P value in the lower energy region of the QD-emission band because the excitons lose their spin polarizations due to the spin relaxation in the dots during the migration. The detailed analysis for the exciton-spin transfer is presented in a coupled QD system after spin injection.

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