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Kim, Nam-Koo,Jang, Soo-Young,Pace, Giuseppina,Caironi, Mario,Park, Won-Tae,Khim, Dongyoon,Kim, Juhwan,Kim, Dong-Yu,Noh, Yong-Young American Chemical Society 2015 Chemistry of materials Vol.27 No.24
<P>In this report, we investigate a formation mechanism for polymer chains aligned with various semiconductor polymers and a microstructure for directionally aligned film through systematic analysis that includes polarized UV–visible–near infrared (UV–vis–NIR) absorption spectroscopy, atomic force microscopy, polarized charge modulation microscopy (<I>p</I>-CMM), and incident X-ray diffraction (GIXD) measurements. Through this study, we make two important observations: first, the highly aligned organic polymer semiconductor films are achieved by off-center spin coating of the preaggregated conjugated polymer solution. Second, the directionally aligned conjugated polymer films exhibit a larger anisotropy on the top surface compared with bulk film, which allows effective mobility improvement in top-gate/bottom-contact field-effect transistors with high performance uniformity. Finally, we demonstrate high-mobility organic field-effect transistors (OFETs) (7.25 cm<SUP>2</SUP>/(V s)) with a mobility large anisotropy (37-fold) using poly[(<I>E</I>)-1,2-(3,3′-dioctadecyl-2,2′- dithienyl)ethylene-<I>alt</I>-dithieno-(3,2-b:2′,3′-d)thiophene] (P18) as the semiconductor layer.</P><P><B>Graphic Abstract</B> <IMG SRC='http://pubs.acs.org/appl/literatum/publisher/achs/journals/content/cmatex/2015/cmatex.2015.27.issue-24/acs.chemmater.5b03775/production/images/medium/cm-2015-03775f_0007.gif'></P><P><A href='http://pubs.acs.org/doi/suppl/10.1021/cm5b03775'>ACS Electronic Supporting Info</A></P>
IUPAC-PSK40: N-Channel Organic Field-Effect Transistors and Structure-Property Relationship
Min Jae Sung,Alessandro Luzio,Won-Tae Park,Ran Kim,Eliot Gann,Francesco Maddalena,Giuseppina Pace,Yong Xu,Dario Natali,Carlo de Falco,Long Dang,Christopher R. McNeill,Mario Caironi,Yong-Young Noh,Yun- 한국고분자학회 2016 한국고분자학회 학술대회 연구논문 초록집 Vol.41 No.2