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Wenwei Yu,Faying Lai,Jinbao He,Kaiyun He,Rong Wang,Danping Li,Quanyuan Chen 한국공업화학회 2023 Journal of Industrial and Engineering Chemistry Vol.118 No.-
Catalytic performances and leaching behavior of 9 natural iron minerals as heterogeneous electro-Fentoncatalysts for the treatment of imidacloprid wastewater were studied. The results showed that magnesioferriteexhibited the best catalytic ability among these minerals with UV absorbance at 270 nm (UV270)removal of 83.59% and COD removal of 49.11% within 4 h using graphite cathode and Ti/(RuO2)0.88-(IrO2)0.12 anode at initial pH 3 with a catalyst dose of 5 g/L, a current density of 40 mA/cm2 and an electrodespacing of 2 cm. The instantaneous current efficiency (ICE) at 4 h and energy consumption (EC)reached 2.30% and 2.20 kWh/gCOD respectively. It was found that the components contained in naturaliron minerals, such as Al, alkali metal (K) and alkaline earth metals (Mg, Ca, Ba), would dissolve into theelectrolyte solution, raising the final pH to 6.5–8.5 and ultimately reducing the reaction efficiency. Exceptmagnetite and magnesioferrite, other minerals, such as ilmenite and V-Ti magnetite, were likely to causesecondary pollution. The subsequent adjustment to alkaline state for chemical precipitation of leachedMn was needed. Pyrite showed relatively high leachability in hazardous elements (especially Pb), whichshould be carefully evaluated before its actual application in electro-Fenton process.
Huantong Liu,Jiang Lai,Lei Sun,Pengzhou Li,Lixia Gao,Danping Yu 한국원자력학회 2019 Nuclear Engineering and Technology Vol.51 No.8
Fluidelastic instability of a tube array is a key factor of the security of a nuclear power plant. An unsteady model of the fluidelastic instability of a tube array subjected to two-phase flow was developed to analyze the fluidelastic instability of tube bundles in two-phase flow. Based on this model, a computational program was written to calculate the eigenvalue and the critical velocity of the fluidelastic instability. The unsteady model and the program were verified by comparing with the experimental results reported previously. The influences of void fraction and the tube's material properties on the critical velocity were investigated. Numerical results showed that, with increasing the void fraction of the two-phase flow, the tube array becomes more stable. The results indicate that the critical velocities of the tube array made of stainless are much higher than those of the other two tube arrays within void fraction ranging from 20%to 80%.