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RISS 인기검색어
- 검색키워드
- 저자 : PAWAN TYAGI (검색결과 3 건)
- 무료
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MOLECULAR SPIN DEVICES: CURRENT UNDERSTANDING AND NEW TERRITORIES
PAWAN TYAGI 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2009 NANO Vol.4 No.6
Molecular spin devices (MSDs) are the most promising candidate for futuristic quantum computation, having potential to resolve spin scattering issue which compromise the utility of conventional spin devices. The MSDs have been extensively reviewed from the view points of device physics and the application of target molecules, such as single molecular magnets. Fabrication of a competent MSD still remains an intractable task. In this review, we first describe the experimental studies where spin state of molecule and/or electrode affected the device transport, especially under magnetic field. Then, we correlated the number of theoretical and experimental results from various domains of nanomagnetism to highlight the scope and future directions panoramically. Finally, the key designs of various MSDs, including our recently developed multilayer edge molecular electrode, have been discussed. A multilayer edge molecular electrode, prepared by bridging the molecular clusters on the exposed edges of a customized ferromagnet–insulator–ferromagnet junction, can be a promising platform for testing the variety of molecular magnets.
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Monte Carlo and Experimental Magnetic Studies of Molecular Spintronics Devices
Pawan Tyagi,Christopher D'Angelo,Collin Baker 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2015 NANO Vol.10 No.4
Molecule-based spintronics devices (MSDs) are highly promising candidates for discovering advanced logic and memory computer units. An advanced MSD will require the placement of paramagnetic molecules between the two ferromagnetic (FM) electrodes. Due to extreme fabrication challenges, only a couple of experimental studies could be performed to understand the effect of magnetic molecules on the overall magnetic and transport properties of MSDs. To date, theoretical studies mainly focused on charge and spin transport aspects of MSDs; there is a dearth of knowledge about the effect of magnetic molecules on the magnetic properties of MSDs. This paper investigates the effect of magnetic molecules, with a net spin, on the magnetic properties of 2D MSDs via Monte Carlo (MC) simulations. Our MC simulations encompass a wide range of MSDs that can be realized by establishing different kinds of magnetic interactions between molecules and FM electrodes at different temperatures. The MC simulations show that ambient thermal energy strongly influenced the molecular coupling effect on the MSD. We studied the nature and strength of molecule couplings (FM and antiferromagnetic) with the two electrodes on the magnetization, specific heat and magnetic susceptibility of MSDs. For the case when the nature of molecule interaction was FM with one electrode and antiferromagnetic with another electrode the overall magnetization shifted toward zero. In this case, the effect of molecules was also a strong function of the nature and strength of direct coupling between FM electrodes. In the case when molecules make opposite magnetic couplings with the two FM electrodes, the MSD model used for MC studies resembled with the magnetic tunnel junction based MSD. The experimental magnetic studies on these devices are in agreement with our theoretical MC simulations results. Our MC simulations will enable the fundamental understanding and designing of a wide range of novel spintronics devices utilizing a variety of molecules, nanoclusters and quantum dots as the device elements.
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Advantages of Prefabricated Tunnel Junction-Based Molecular Spintronics Devices
Pawan Tyagi,Edward Friebe,Collin Baker 성균관대학교(자연과학캠퍼스) 성균나노과학기술원 2015 NANO Vol.10 No.4
Molecule-based devices may govern the advancement of the next generation's logic and memory devices. Molecules have the potential to be unmatched device elements as chemists can mass produce an endless variety of molecules with novel optical, magnetic and charge transport characteristics. However, the biggest challenge is to connect two metal leads to a target molecule (s) and develop a robust and versatile device fabrication technology that can be adopted for commercial scale mass production. This paper discusses distinct advantages of utilizing commercially successful tunnel junctions as a vehicle for developing molecular spintronics devices. We describe the use of a prefabricated tunnel junction with the exposed sides as a testbed for molecular device fabrication. On the exposed sides of a tunnel junction molecules are bridged across an insulator by chemically bonding with the two metal electrodes; sequential growth of metal–insulator–metal layers ensures that separation between two metal electrodes is controlled by the insulator thickness to the molecular device length scale. This paper highlights various attributes of tunnel junction-based molecular devices with ferromagnetic electrodes for making molecular spintronics devices. We strongly emphasize a need for close collaboration between chemists and magnetic tunnel junction (MTJ) researchers. Such partnerships will have a strong potential to develop tunnel junction-based molecular devices for futuristic areas such as memory devices, magnetic metamaterials, high sensitivity multi-chemical biosensors, etc.
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