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He Binhong,Wen Shuntao,Wen Zhiming,Liang Yan,Yang Qianxi,Zhou Minjie,Wang Wei,Wang Guo-Xiang 한국탄소학회 2024 Carbon Letters Vol.34 No.3
This paper reports an enhanced strategy for improving the mechanical flexibility and ionic kinetic properties of a double network hydrogel based on Co2+-coordination assistance. The modified double-network hydrogel was obtained by using acrylic acid and N, N-dimethylacrylamide as monomers, adding cross-linking agents and 3D nitrogen-doped graphenes. The tensile fracture rate of the modified hydrogel was 1925% and its tensile strength was 1696 kPa. In addition, the hydrogel exhibited excellent ionic dynamics, and its application to an all-solid-state supercapacitor was able to achieve a specific capacitance of up to 182.8 F g−1. The supercapacitor exhibited an energy density of 34.2 Wh kg−1, even when operating at a power density of 5 kW kg−1, highlighting its significant potential for practical applications.
Danyang Han,Guo Yu,An Liu,Gangyong Li,Wei Wang,Binhong He,Zhaohui Hou,Hong Yin 한국탄소학회 2023 Carbon Letters Vol.33 No.6
As a promising anode for sodium-ion batteries (SIBs), cobalt sulfide ( CoS2) has attracted extensive attention due to its high theoretical capacity, easy preparation, and superior electrochemical activity. However, its intrinsic low conductivity and large volume expansion result in poor cycling ability. Herein, nitrogen-doped carbon-coated CoS2 nanoparticles (N–C@ CoS2) were prepared by a C3N4 soft-template-assisted method. Carbon coating improves the conductivity and prevents the aggregation of CoS2 nanoparticles. In addition, the C3N4 template provides a porous graphene-like structure as a conductive framework, affording a fast and constant transport path for electrons and void space for buffering the volume change of CoS2 nanoparticles. Benefitting from the superiorities, the Na-storage properties of the N–C@CoS2 electrode are remarkably boosted. The advanced anode delivers a long-term capacity of 376.27 mAh g? 1 at 0.1 A g? 1 after 500 cycles. This method can also apply to preparing other metal sulfide materials for SIBs and provides the relevant experimental basis for the further development of energy storage materials.
Qinghua Wang,Wei Wang,Junlin Huang,Hong Yin,Yucan Zhu,Haitao Wang,Minjie Zhou,Binhong He,Zhaohui Hou,Wenyuan Xu 한국탄소학회 2023 Carbon Letters Vol.33 No.1
Transition-metal phosphides (TMPs), a promising anode material for lithium-ion batteries (LIBs), are limited in application because of its serious volume effect in the cycle. In this work, a simple electrospinning strategy was proposed to restrict the grain size of CoP nanocrystals by nano-confined effect of carbon nanofibers with ligands. The addition of ligands not only could realize the uniform dispersion of CoP nanocrystals, but also strengthen the bond between the metals and carbon nanofibers. As a result, the CoP/CNF composite exhibits excellent lithium storage performance, and its reversible specific capacity could reach 1016.4 mAh g? 1 after 200 cycles at a current density of 200 mA g? 1. The research is anticipated to provide a new idea for the preparation of anode materials for lithium ion batteries.