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Effect of Linear Chirp on Strong Field Photodissociation of H_2^+
Vaibhav S. Prabhudesai,Adi Natan,Barry D. Bruner,Yaron Silberberg,Uri Lev,Oded Heber,Daniel Strasser,Dirk Schwalm,Daniel Zajfman,Itzik Ben-Itzhak 한국물리학회 2011 THE JOURNAL OF THE KOREAN PHYSICAL SOCIETY Vol.59 No.41
We report the experimental findings of a systematic study of the effect of the linear chirp on strong field photodissociation of H_2^+. For vibrational levels around or above the one photon crossing, the effect manifests in terms of a shift in the kinetic energy release (KER) peaks. The peaks shift up for negative chirp whereas they shift down for positive chirp. The measurements are carried out by varying two of the laser pulse characteristics energy, pulse intensity and linear chirp while keeping the third constant. The shifts in the KER peaks are found to be intensity dependent for a given value of chirp. However, in the last two cases, they are found to be independent of the chirp magnitude. The results are understood on the basis of saturation of photodissociation probabilities for these levels.