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      키틴과 헥사시아노페레이트 복합체를 이용한 수용액 중 세슘 제거 = Removal of Cs(I) Ions in Aqueous Solution by Chitin and Hexacyanoferrate Compounds

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      https://www.riss.kr/link?id=A106051196

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      다국어 초록 (Multilingual Abstract)

      Recently, the nuclear accident of Fukushima in Japan has caused many radioactive materials to leak into the sea and the interest in the disposal of radioactive pollutants in the world is getting bigger. Thus, effective treatment techniques for removing radioactive ions in water are needed. In this study, chitin was used to remove Cs(I) in water. Chitin, hexacyanoferrate and CuCl2 were synthesized and adsorbent (CuHCF) was prepared and used for characterization and batch experiments. SEM / EDX and XRD analysis confirmed the K, Fe and Cu synthesis of CuHCF. Batch experiments were performed by pH, time, and initial concentration. The removal of CuHCF was 1.5 times higher than chitin. As a result of the time experiment, all of the three adsorbents reached equilibrium after 300 minutes and the optimum time was set to 300 minutes. As a result of the isothermal adsorption experiments on Cs(I), the maximum adsorption quantity of chitin and CuHCF were 2.72 mg/g and 18.5 mg/g and CuHCF was about 6 times higher than chitin. Chtin and CuHCF were found to be specific adsorbents which were not influenced by ionic strength. As a result, CuHCF modified with chitin and Cu and HCF could be used as an adsorbent for the efficient treatment of wastewater contaminated with Cs(I).
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      Recently, the nuclear accident of Fukushima in Japan has caused many radioactive materials to leak into the sea and the interest in the disposal of radioactive pollutants in the world is getting bigger. Thus, effective treatment techniques for removin...

      Recently, the nuclear accident of Fukushima in Japan has caused many radioactive materials to leak into the sea and the interest in the disposal of radioactive pollutants in the world is getting bigger. Thus, effective treatment techniques for removing radioactive ions in water are needed. In this study, chitin was used to remove Cs(I) in water. Chitin, hexacyanoferrate and CuCl2 were synthesized and adsorbent (CuHCF) was prepared and used for characterization and batch experiments. SEM / EDX and XRD analysis confirmed the K, Fe and Cu synthesis of CuHCF. Batch experiments were performed by pH, time, and initial concentration. The removal of CuHCF was 1.5 times higher than chitin. As a result of the time experiment, all of the three adsorbents reached equilibrium after 300 minutes and the optimum time was set to 300 minutes. As a result of the isothermal adsorption experiments on Cs(I), the maximum adsorption quantity of chitin and CuHCF were 2.72 mg/g and 18.5 mg/g and CuHCF was about 6 times higher than chitin. Chtin and CuHCF were found to be specific adsorbents which were not influenced by ionic strength. As a result, CuHCF modified with chitin and Cu and HCF could be used as an adsorbent for the efficient treatment of wastewater contaminated with Cs(I).

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      참고문헌 (Reference)

      1 이민규, "활성탄에 의한 난분해성 염료인 Eosin Y의 흡착" 한국환경과학회 21 (21): 623-631, 2012

      2 박광하, "키틴에 의한 중금속 Cd(Ⅱ), Pb(Ⅱ)이온의 흡착 및 회수에 관한 연구" 한국분석과학회 15 (15): 163-171, 2002

      3 이창한, "제올라이트 NaX에 의한 방사성 물질인 Cs 이온의 흡착 특성" 대한환경공학회 39 (39): 66-73, 2017

      4 이창한, "스트론튬과 세슘 이온의 혼합 몰비를 달리한 이성분 용액에서 제올라이트 A에 의한 경쟁 흡착: 흡착등온 및 속도해석" 한국환경과학회 24 (24): 151-162, 2015

      5 정우창, "수중의 세슘처리를 위한 수처리 기술 동향 및 개선방안" 한국수처리학회 25 (25): 99-114, 2017

      6 Su, J., Y., "The characterization and application of prussian blue at graphene coated carbon fibers in a separated adsorption and electrically switched ion exchange desorption processes of cesium" 230 : 399-406, 2017

      7 Vipin, A. K, "Sodium Cobalt Hexacynoferrate Encapsulated in Alginate Vesicle with CNT for both Cesium and Strontium Removal" 111 : 477-484, 2014

      8 Sangvanich, T, "Selective capture of cesium and thalliumfrom natural waters and simulated wastes with copper ferrocyanide function-alized mesoporous silica" 182 : 225-231, 2010

      9 Clarke, T. D., "Selective Removal of Ce\-sium from Acid Solutions with Immobilized Copper Ferrocyanide" 70 : 3708-3711, 1998

      10 Dubourg, M., "Review of Advanced Methods for Treating Radioactive Contaminated Water" 33 (33): 35-46, 1998

      1 이민규, "활성탄에 의한 난분해성 염료인 Eosin Y의 흡착" 한국환경과학회 21 (21): 623-631, 2012

      2 박광하, "키틴에 의한 중금속 Cd(Ⅱ), Pb(Ⅱ)이온의 흡착 및 회수에 관한 연구" 한국분석과학회 15 (15): 163-171, 2002

      3 이창한, "제올라이트 NaX에 의한 방사성 물질인 Cs 이온의 흡착 특성" 대한환경공학회 39 (39): 66-73, 2017

      4 이창한, "스트론튬과 세슘 이온의 혼합 몰비를 달리한 이성분 용액에서 제올라이트 A에 의한 경쟁 흡착: 흡착등온 및 속도해석" 한국환경과학회 24 (24): 151-162, 2015

      5 정우창, "수중의 세슘처리를 위한 수처리 기술 동향 및 개선방안" 한국수처리학회 25 (25): 99-114, 2017

      6 Su, J., Y., "The characterization and application of prussian blue at graphene coated carbon fibers in a separated adsorption and electrically switched ion exchange desorption processes of cesium" 230 : 399-406, 2017

      7 Vipin, A. K, "Sodium Cobalt Hexacynoferrate Encapsulated in Alginate Vesicle with CNT for both Cesium and Strontium Removal" 111 : 477-484, 2014

      8 Sangvanich, T, "Selective capture of cesium and thalliumfrom natural waters and simulated wastes with copper ferrocyanide function-alized mesoporous silica" 182 : 225-231, 2010

      9 Clarke, T. D., "Selective Removal of Ce\-sium from Acid Solutions with Immobilized Copper Ferrocyanide" 70 : 3708-3711, 1998

      10 Dubourg, M., "Review of Advanced Methods for Treating Radioactive Contaminated Water" 33 (33): 35-46, 1998

      11 Chegrouche, S., "Removal of strontium from aqueous solutions by adsorption onto activated carbon: kinetic and thermodynamic studies" 235 (235): 306-318, 2009

      12 Choong Jeon, "Removal of lead ions using phosphorylated sawdust" 한국공업화학회 15 (15): 910-913, 2009

      13 전충, "Removal of cesium ion in aqueous solution using immobilized sericite beads" 한국화학공학회 31 (31): 1219-1224, 2014

      14 이창한, "Polysulfone으로 제올라이트 A를 고정화한 방사성 물질제거용 PS-zeolite 비드 제조" 대한환경공학회 37 (37): 145-151, 2015

      15 이창한, "PVC-Zeolite 복합체에 의한 수용액 중의 Sr 이온과 Cs 이온의 제거" 한국환경과학회 24 (24): 1145-1153, 2015

      16 Cetina, M., "Modelling of circulation and dispersion ofradioactive pollutants in the Japan Sea" 23 : 819-836, 2000

      17 Krestou, A., "Mechanism of aqueous uranium (VI) uptake by natural zeolitic tuff" 16 (16): 1363-1370, 2003

      18 Babel, S., "Low-cost adsorbents for heavy metals uptake from contaminated water: a review" 97 : 219-243, 2003

      19 Ofomaja, A. E., "Kinetics and competitive modeling ofcesium biosorption onto iron(III)hexacyanoferrate modified pine cone powder" 92 : 71-78, 2014

      20 Zhang, Z., "Kinetic and thermodynamic analysis of selective adsorption of Cs(I) by a novel surface whisker-supported ion-imprinted polymer" 263 : 97-, 2010

      21 Cappelletti, P, "Immobiliztion of Cs and Sr in Aluminosilicate Matrices Derived from Natural Zeolites" 414 : 451-457, 2011

      22 Lalhmunsiama, Lalhriatpuia, C., "Immobilized nickel hexacyanoferrate on activated carbons for efficient attenuation of radio toxic Cs(I)from aqueous solutions" 321 : 275-282, 2014

      23 Yi, R, "Highly efficient removal of 137Cs in seawater by potassium titanium ferrocyanide functionalized magnetic microspheres with multilayer core-shell structure" 4 : 37600-37608, 2014

      24 Leppert, D., "Heavy metal sorption with clinoptilolite zeolite: alternatives for treating contaminated soil and water" 42 (42): 604-608, 1990

      25 Yang, J. G., "Heavy metal removal and crude bio-oil upgrading from Sedum plumbizincicola harvest using hydrothermal upgrading process" 101 (101): 7653-7657, 2010

      26 International Atomic Energy Agency, "Handing and Treatment of Radioactive Aqueous Wastes" IAEA 654-, 1992

      27 Pawar, R. R, "Efficient removal of hazardous lead, cadmium, and arsenic from aqueous environment by iron oxide modified clay-activated carbon composite beads" 162 : 339-350, 2018

      28 Yu, W, "Distribution and risk assessment of radionuclides released by Fukushima nuclear accident at the northwest Pacific" 142 : 54-61, 2015

      29 Yu, B, "Crystalline Silicotitanate : A New Type of Ion Exchanger for Cs Removal from Liquid Waste" 18 (18): 206-210, 2002

      30 Vincent, C., "Chitin-Prussian blue sponges for Cs(I) recovery: From synthesis to application in the treatment of accidental dumping of metal-bearing solutions" 287 : 171-179, 2015

      31 Ghaemi, A., "Characterizations ofstrontium(II) and barium(II) adsorption from aqueous solutions using dolomitepowder" 190 : 916-921, 2011

      32 Mobtaker, H, "Cesium removal from nuclear waste using a magnetical CuHCNPAN nano composite" 482 : 306-312, 2016

      33 이청호, "Arsenate and phosphate removal from water using Fe-sericite composite beads in batch and fixed-bed systems" 한국공업화학회 47 : 375-383, 2017

      34 Ding, D, "Adsorption ofcesium from aqueous solution using agricultural residue-walnut shell:equilibrium, kinetic and thermodynamic mode-ling studies" 47 : 2563-2571, 2013

      35 Soco, E, "Adsorption of nickel(II) and copper(II) ions from aqueous solution by coal fly ash" 1 (1): 581-588, 2013

      36 Ding, D, "Adsorption of cesium from aqueous solution using agricultural residue-Walnut shell:Equilibrium, kinetic and thermodynamic modeling studies" 47 (47): 2563-2571, 2013

      37 Ding, D, "Adsorption of cesium from aqueous solution using agricultural residue-Walnut shell:Equilibrium, kinetic and thermodynamic modeling studies" 47 (47): 2563-2571, 2013

      38 Kim, J. O, "Adsorption characteristics of sericite for cesium ions from an aqueous solution" 92 : 368-374, 2014

      39 Dechojarassri, D., "Adsorption and desorption behaviors of cesium on rayon fibers coated with chitosan immobilized with Prussian blue" 104 : 1509-1516, 2017

      40 Saberi, R, "Adsorption Characteristic of 137Cs from Aqueous Solution Using PAN-Based Sodium Titanosilicate Composite" 284 : 461-469, 2010

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