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      KCI등재 SCOPUS SCIE

      Controlling spin-orbit coupling strength of bulk transition metal dichalcogenide semiconductors

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      https://www.riss.kr/link?id=A107900195

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      다국어 초록 (Multilingual Abstract)

      Transition metal dichalcogenide (TMD) semiconductors are attracting much attention in research regarding device physics based on their unique properties that can be utilized in spintronics and valleytronics. Although current studies concentrate on the monolayer form due to the explicitly broken inversion symmetry and the direct band gap, bulk materials also hold the capability of carrying spin and valley current. In this study, we report the methodology to continuously control the spin-orbit coupling (SOC) strength of bulk TMDs Mo1-xWxSe2 by changing the atomic ratio between Mo and W. The results show the size of band splitting at the K valley the measure of the coupling strength is linearly proportional to the atomic ratio of Mo and W. Our results thus demonstrate how to precisely tune the SOC coupling strength, and the collected information of which can serve as a reference for future applications of bulk TMDs.
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      Transition metal dichalcogenide (TMD) semiconductors are attracting much attention in research regarding device physics based on their unique properties that can be utilized in spintronics and valleytronics. Although current studies concentrate on the...

      Transition metal dichalcogenide (TMD) semiconductors are attracting much attention in research regarding device physics based on their unique properties that can be utilized in spintronics and valleytronics. Although current studies concentrate on the monolayer form due to the explicitly broken inversion symmetry and the direct band gap, bulk materials also hold the capability of carrying spin and valley current. In this study, we report the methodology to continuously control the spin-orbit coupling (SOC) strength of bulk TMDs Mo1-xWxSe2 by changing the atomic ratio between Mo and W. The results show the size of band splitting at the K valley the measure of the coupling strength is linearly proportional to the atomic ratio of Mo and W. Our results thus demonstrate how to precisely tune the SOC coupling strength, and the collected information of which can serve as a reference for future applications of bulk TMDs.

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      참고문헌 (Reference)

      1 T. Cao, "Valley-selective circular dichroism of molybdenum disulphide" 3 : 887-, 2012

      2 H. Zeng, "Valley polarization in MoS2 monolayers by optical pumping" 7 : 490-493, 2012

      3 M. Kang, "Universal mechanism of band-gap engineering in transition-metal dichalcogenides" 17 (17): 1610-1615, 2017

      4 Mei Zhang, "Two-Dimensional Molybdenum Tungsten Diselenide Alloys: Photoluminescence, Raman Scattering, and Electrical Transport" American Chemical Society (ACS) 8 (8): 7130-7137, 2014

      5 Won Seok Yun, "Thickness and strain effects on electronic structures of transition metal dichalcogenides: 2H- M X 2 semiconductors ( M = Mo, W; X = S, Se, Te)" American Physical Society (APS) 85 (85): 2012

      6 S. B. Desai, "Strain-induced indirect to direct bandgap transition in multilayer WSe2" 14 (14): 4592-4597, 2014

      7 G. Wang, "Spin-orbit engineering in transition metal dichalcogenide alloy monolayers" 6 : 10110-, 2015

      8 Xiaodong Xu, "Spin and pseudospins in layered transition metal dichalcogenides" Springer Science and Business Media LLC 10 (10): 343-350, 2014

      9 Y. K. Luo, "Opto-valleytronic spin injection on monolayer MoS2/few-layer graphene hybrid spin valves" 17 (17): 3877-3883, 2017

      10 Nasser Alidoust, "Observation of monolayer valence band spin-orbit effect and induced quantum well states in MoX2" Springer Science and Business Media LLC 5 (5): 4673-, 2014

      1 T. Cao, "Valley-selective circular dichroism of molybdenum disulphide" 3 : 887-, 2012

      2 H. Zeng, "Valley polarization in MoS2 monolayers by optical pumping" 7 : 490-493, 2012

      3 M. Kang, "Universal mechanism of band-gap engineering in transition-metal dichalcogenides" 17 (17): 1610-1615, 2017

      4 Mei Zhang, "Two-Dimensional Molybdenum Tungsten Diselenide Alloys: Photoluminescence, Raman Scattering, and Electrical Transport" American Chemical Society (ACS) 8 (8): 7130-7137, 2014

      5 Won Seok Yun, "Thickness and strain effects on electronic structures of transition metal dichalcogenides: 2H- M X 2 semiconductors ( M = Mo, W; X = S, Se, Te)" American Physical Society (APS) 85 (85): 2012

      6 S. B. Desai, "Strain-induced indirect to direct bandgap transition in multilayer WSe2" 14 (14): 4592-4597, 2014

      7 G. Wang, "Spin-orbit engineering in transition metal dichalcogenide alloy monolayers" 6 : 10110-, 2015

      8 Xiaodong Xu, "Spin and pseudospins in layered transition metal dichalcogenides" Springer Science and Business Media LLC 10 (10): 343-350, 2014

      9 Y. K. Luo, "Opto-valleytronic spin injection on monolayer MoS2/few-layer graphene hybrid spin valves" 17 (17): 3877-3883, 2017

      10 Nasser Alidoust, "Observation of monolayer valence band spin-orbit effect and induced quantum well states in MoX2" Springer Science and Business Media LLC 5 (5): 4673-, 2014

      11 J. M. Riley, "Negative electronic compressibility and tunable spin splitting in WSe2" Springer Science and Business Media LLC 10 (10): 1043-1047, 2015

      12 Z. Y. Zhu, "Giant spin-orbit-induced spin splitting in two-dimensional transition-metal dichalcogenide semiconductors" 84 : 153402-, 2011

      13 Hongtao Yuan, "Generation and electric control of spin–valley-coupled circular photogalvanic current in WSe2" Springer Science and Business Media LLC 9 (9): 851-857, 2014

      14 Yi Zhang, "Electronic Structure, Surface Doping, and Optical Response in Epitaxial WSe 2 Thin Films" American Chemical Society (ACS) 16 (16): 2485-2491, 2016

      15 Y. Zhang, "Direct observation of the transition from indirect to direct bandgap in atomically thin epitaxial MoSe2" 9 : 111-115, 2014

      16 J. M. Riley, "Direct observation of spin-polarized bulk bands in an inversion-symmetric semiconductor" 10 : 835-839, 2014

      17 Beom Seo Kim, "Determination of the band parameters of bulk 2H-MX2 (M = Mo, W; X = S, Se) by angle-resolved photoemission spectroscopy" Springer Science and Business Media LLC 6 (6): 36389-, 2016

      18 K. F. Mak, "Control of valley polarization in monolayer MoS2 by optical helicity" 10 : 494-498, 2012

      19 Y. -H. Zhao, "Continuously tunable electronic structure of transition metal dichalcogenides superlattices" 5 : 8356-, 2015

      20 S. Manzeli, "2D transition metal dichalcogenides" 2 : 17033-, 2017

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      2023 평가예정 해외DB학술지평가 신청대상 (해외등재 학술지 평가)
      2020-01-01 평가 등재학술지 유지 (해외등재 학술지 평가) KCI등재
      2008-01-01 평가 등재학술지 선정 (등재후보2차) KCI등재
      2007-01-01 평가 등재후보 1차 PASS (등재후보1차) KCI등재후보
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      기준연도 WOS-KCI 통합IF(2년) KCIF(2년) KCIF(3년)
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      KCIF(4년) KCIF(5년) 중심성지수(3년) 즉시성지수
      0.92 0.77 0.297 0.1
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