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      KCI등재 SCOPUS SCIE

      Correlation between pit formation and phase separation in thick InGaN film on a Si substrate

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      https://www.riss.kr/link?id=A105960096

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      다국어 초록 (Multilingual Abstract)

      We demonstrate improved surface pit and phase separation in thick InGaN grown on a GaN/Si (111) substrate, using plasma-assisted molecular beam epitaxy with an indium modulation technique. The formation of surface pit and compositional inhomogeneity in the InGaN epilayer are investigated using atomic force microscopy, scanning electron microscopy and temperature-dependent photoluminescence. Indium elemental mapping directly reveals that poor compositional homogeneity occurs near the pits. The indium-modulation epitaxy of InGaN minimizes the surface indium segregation, leading to the reduction in pit density and size. The phase separation in InGaN with a higher pit density is significantly suppressed, suggesting that the pit formation and the phase separation are correlated.
      We propose an indium migration model for the correlation between surface pit and phase separation in InGaN.
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      We demonstrate improved surface pit and phase separation in thick InGaN grown on a GaN/Si (111) substrate, using plasma-assisted molecular beam epitaxy with an indium modulation technique. The formation of surface pit and compositional inhomogeneity i...

      We demonstrate improved surface pit and phase separation in thick InGaN grown on a GaN/Si (111) substrate, using plasma-assisted molecular beam epitaxy with an indium modulation technique. The formation of surface pit and compositional inhomogeneity in the InGaN epilayer are investigated using atomic force microscopy, scanning electron microscopy and temperature-dependent photoluminescence. Indium elemental mapping directly reveals that poor compositional homogeneity occurs near the pits. The indium-modulation epitaxy of InGaN minimizes the surface indium segregation, leading to the reduction in pit density and size. The phase separation in InGaN with a higher pit density is significantly suppressed, suggesting that the pit formation and the phase separation are correlated.
      We propose an indium migration model for the correlation between surface pit and phase separation in InGaN.

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      참고문헌 (Reference)

      1 Y. -H. Cho, "“S-shaped” temperature-dependent emission shift and Carrier dynamics in InGaN/GaN multiple quantum wells" 73 : 1370-, 1998

      2 Y. Narukawa, "of self-formed InGaN quantum dots for exciton localization in the purple laser diode emitting at 420 nm" 70 : 981-, 1997

      3 K. Hiramatsu, "The composition pulling effect in MOVPE grown InGaN on GaN and AlGaN and its TEM characterization" 2 : 6-, 1997

      4 Y. P. Varshni, "Temperature dependence of the energy gap in semiconductors" 34 : 149-, 1967

      5 F. B. Nranjo, "Structural and optical characterization of thick InGaN layers and InGaN/GaN MQW grown by molecular beam epitaxy" 93 : 131-134, 2002

      6 F. Bertram, "Spatial variation of luminescence of InGaN alloys measured by highly-spatially-resolved scanning cathodoluminescence" 93 : 19-23, 2002

      7 P. R. Edwards, "Simultaneous composition mapping and hyperspectral cathodoluminescence imaging of InGaN epilayers" 0 : 2474-2477, 2003

      8 Y. S. Park, "Photoluminescence studies of GaN nanorods on Si (111) substrates grown by molecular-beam epitaxy" 85 : 5718-, 2004

      9 우현석, "Phase separation suppression in InxGa1 xN on a Si substrate using an indium modulation technique" 한국물리학회 17 (17): 1142-1147, 2017

      10 C. A. Tran, "Phase separation in InGaN/GaN multiple quantum wells and its relation to brightness of blue and green LEDs" 195 : 397-400, 1998

      1 Y. -H. Cho, "“S-shaped” temperature-dependent emission shift and Carrier dynamics in InGaN/GaN multiple quantum wells" 73 : 1370-, 1998

      2 Y. Narukawa, "of self-formed InGaN quantum dots for exciton localization in the purple laser diode emitting at 420 nm" 70 : 981-, 1997

      3 K. Hiramatsu, "The composition pulling effect in MOVPE grown InGaN on GaN and AlGaN and its TEM characterization" 2 : 6-, 1997

      4 Y. P. Varshni, "Temperature dependence of the energy gap in semiconductors" 34 : 149-, 1967

      5 F. B. Nranjo, "Structural and optical characterization of thick InGaN layers and InGaN/GaN MQW grown by molecular beam epitaxy" 93 : 131-134, 2002

      6 F. Bertram, "Spatial variation of luminescence of InGaN alloys measured by highly-spatially-resolved scanning cathodoluminescence" 93 : 19-23, 2002

      7 P. R. Edwards, "Simultaneous composition mapping and hyperspectral cathodoluminescence imaging of InGaN epilayers" 0 : 2474-2477, 2003

      8 Y. S. Park, "Photoluminescence studies of GaN nanorods on Si (111) substrates grown by molecular-beam epitaxy" 85 : 5718-, 2004

      9 우현석, "Phase separation suppression in InxGa1 xN on a Si substrate using an indium modulation technique" 한국물리학회 17 (17): 1142-1147, 2017

      10 C. A. Tran, "Phase separation in InGaN/GaN multiple quantum wells and its relation to brightness of blue and green LEDs" 195 : 397-400, 1998

      11 D. Doppalapudi, "Phase separation and ordering in InGaN alloys grown by molecular beam epitaxy" 84 : 1389-, 1998

      12 E. -L. Lai, "Origins of efficient green light emission in phase-separated InGaN quantum wells" 17 : 3734-3739, 2006

      13 P. Mishra, "On the optical and microstrain analysis of graded InGaN/GaN MQWs based on plasma assisted molecular beam epitaxy" 6 : 2052-2062, 2016

      14 M. Moseley, "Observation and control of the surface kinetics of InGaN for the elimination of phase separation" 112 : 014909-, 2012

      15 A. Lotsari, "Morphology and origin of V-defects in semipolar (11–22) InGaN" 339 : 1-7, 2012

      16 S. Chichibu, "Luminescences from localized states in InGaN epilayers" 70 : 2822-, 1997

      17 T. Kimura, "Investigation of InN mole fraction fluctuation in InGaN films grown by RF-MBE" 8 : 1499-1502, 2011

      18 S. Nakamura, "Introduction to Nitride Semiconductor Blue Lasers and Light Emitting Diodes" CRC Press 2000

      19 Th Kehagias, "Indium migration paths in V-defects of InAlN grown by metal-organic vapor phase epitaxy" 95 : 071905-, 2009

      20 J. Bruckbauer, "High resolution cathodoluminescence hyperspectral imaging of surface features in InGaN/GaN multiple quantum well structures" 98 : 141908-, 2011

      21 A. Yamamoto, "Growth temperature dependent critical thickness for phase separation in thick(~1 μm)InxGa1−xN(x=0. 2–0. 4)" 419 : 64-68, 2015

      22 B. N. Pantha, "Evolution of phase separation in In-rich InGaN alloys" 96 : 232105-, 2010

      23 I. -K. Park, "Enhancement of phase separation in the InGaN layer for selfassembled In-rich quantum dots" 87 : 061906-, 2005

      24 A. Chakraborty, "Elimination of Vshaped pits in InGaN/GaN/AlN/GaN heterostructure by metal modulation growth technique" 33 : 035009-, 2018

      25 H. Woo, "Effect of heating on electrical transport in AlGaN/GaN Schottky barrier diodes on Si substrate" 14 : S98-S102, 2014

      26 C. Bazioti, "Dimitrakopulos, Defects, strain relaxation, and compositional grading in high indium content InGaN epilayers grown by molecular beam epitaxy" 118 : 155301-, 2005

      27 우현석, "Barrier lowering and leakage current reduction in Ni-AlGaN/GaN Schottky diodes with an oxygen-treated GaN cap layer" 한국물리학회 15 (15): 1027-2031, 2015

      28 S. Y. Woo, "Atomic ordering in InGaN alloys within nanowire heterostructures" 15 : 6413-, 2015

      29 S. Srinivasan, "A comparison of Rutherford Backscattering spectroscopy and X‐ray diffraction to determine the composition of thick InGaN epilayers" 228 : 41-44, 2001

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